2020
DOI: 10.1002/adfm.201908993
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Enhanced Sensitivity of Iontronic Graphene Tactile Sensors Facilitated by Spreading of Ionic Liquid Pinned on Graphene Grid

Abstract: Iontronic graphene tactile sensors (i‐GTS) composed of a top floating graphene electrode and an ionic liquid droplet pinned on a bottom graphene grid, which can dramatically enhance the performance of capacitive‐type tactile sensors, are presented. When mechanical stress is applied to the top floating electrode, the i‐GTS operates in one of the following three regimes: air–air, air–electric double layer (EDL) transition, or EDL–EDL. Once the top electrode contacts the ionic liquid in the i‐GTS, the spreading b… Show more

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Cited by 40 publications
(22 citation statements)
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“…For instance, Guo et al achieved a graded intrafillable architecture-based iontronic PPS with unprecedently high sensitivity ( S min > 220 kPa −1 ) and a broad pressure regime (0.08 Pa–360 kPa) [ 23 ]. Kim et al developed the top floating electrode for iontronic PPS with greatly enhanced sensitivity [ 20 ]. Additionally, recently introducing the remarkable interfacial capacitance for PPS by electrical double layer (EDL) effect is also an effective strategy [ 24 ].…”
Section: Introductionmentioning
confidence: 99%
See 1 more Smart Citation
“…For instance, Guo et al achieved a graded intrafillable architecture-based iontronic PPS with unprecedently high sensitivity ( S min > 220 kPa −1 ) and a broad pressure regime (0.08 Pa–360 kPa) [ 23 ]. Kim et al developed the top floating electrode for iontronic PPS with greatly enhanced sensitivity [ 20 ]. Additionally, recently introducing the remarkable interfacial capacitance for PPS by electrical double layer (EDL) effect is also an effective strategy [ 24 ].…”
Section: Introductionmentioning
confidence: 99%
“…Additionally, recently introducing the remarkable interfacial capacitance for PPS by electrical double layer (EDL) effect is also an effective strategy [ 24 ]. For example, Pan et al introduced the iontronic PPS based on the EDL capacitive materials [ 21 , 25 , 26 ], such as graphene [ 20 ], silver [ 21 ], and Au [ 23 ]. Thanks to its high areal capacitance (up to nF or even near µF), the EDL-based iontronic sensor showed much higher sensitivity and broader sensing range than traditional PPS.…”
Section: Introductionmentioning
confidence: 99%
“…Compared to conventional capacitive sensors, supercapacitive interfacial IFS based on an EDL can produce an ultrahigh capacitance per unit area up to several µF cm −2 in the sub-MHz spectrum, where the capacitive value increased by more than 1000 times. [30] Generally, the electrode with excess carriers will generate strong electrostatic force. When the ionic material (solid or liquid) contacts the electronic conductor (electrode), the charged electronic conductor will repel the ions with the same charge, whereas the ions with opposite charge are attracted to the electrode surface.…”
Section: Supercapacitive Interface Effectmentioning
confidence: 99%
“…The GO/GO foam‐based capacitive pressure sensor demonstrated a pressure detection limit of ≈0.24 Pa with high sensitivity (≈0.8 kPa −1 ), outperforming GO‐based capacitive pressure sensors using PDMS [ 650,661 ] or air [ 662 ] as the dielectric. Kim et al [ 663 ] designed a novel iontronic graphene tactile sensor, which consisted of a top float graphene electrode and an ionic liquid droplet pinned on the bottom graphene grid. Under external pressure, the ionic liquid rapidly spreads out, causing a capacitance transition (from several pF to more than hundreds of pF) to form an air‐electric double layer at the interface.…”
Section: D Materials‐based Wearable Sensors For Human Health Applicationsmentioning
confidence: 99%