Laser Polishing (LP) is a well-defined technology that has recently been applied to improve three-dimensional (3D) printed Inconel 718 (IN718) parts. However, the necessity to conduct the process in an argon chamber is one of its major drawbacks, which is associated with an increase in the costs of production and the limitations of the technology regarding the size of parts that can be polished. This article investigates the possibility to conduct LP of IN718 in an air atmosphere and compares the results with those from an argon chamber setup. The experiment was carried out in the context of the influence of overlap on the final surface. The improvement of surface quality was defined through the evaluation of average areal roughness parameters, material relocation, periodic surface components, and the categorization of process-induced structures. It was found that LP allows for the average roughness to be reduced by 82.8% and 87.9% for an air and argon atmosphere, respectively. The oxidation layer was characterized using Energy-Dispersive X-ray Spectroscopy (EDS) analysis. The formation of overlap with regards to Ti and Al oxides had a vital influence on surface quality.