“…Devices based on transition metal oxides, such as NiO x , 2-4 TiO x , 4,5 HfO x , 6 Ta 2 O 5 , 5,7,8 and SiO x , 9,10 have all demonstrated resistive switching with some devices exhibiting resistance ratios and cycling endurances sufficient for many computational memory applications. 9,[11][12][13][14][15][16] Resistive switching in oxide-based systems is thought to arise from the rupture and reformation of nanoscale conducting filaments that span the oxide. 1,4,13,[17][18][19] A fully formed, intact filament yields the conductive LRS, while a ruptured filament leads to the HRS.…”