“…[12][13][14] Surface plasmons (SPs) with field E SP excited by an incoming light E 0 can enhance fluorophore excitation rate and Raman scattering by factors up to |E sp /E 0 | 2 and |E sp /E 0 | 4 , respectively. [15][16][17][18] Various metal nanostructures have been reported for the enhancement of fluorescence emission, such as nanoholes, [19][20][21] nanorods, 22,23 core-shell nanoparticles, [24][25][26] bowtie nanoantennas, 27,28 DNA-assembled nanoparticles, 29 and antennas-in-box. 30 The SPFS based on metallic thin film is usually achieved with Kretschmann configuration by coupling evanescent waves with SPs, which has been reported for highly sensitive detection of biomolecules including biomarkers, 31,32 toxins, and oligonucleotides, 33 with the limit of detection (LOD) down to attomolar range.…”