“…However, the zero-bandgap structure limits its advanced application as optoelectronic devices. Subsequently, inspired by graphene, 2D materials including topological insulators (TIs) [13][14][15][16][17], transition metal dichalcogenides (TMDs) [18][19][20][21][22][23][24][25][26] and black phosphorus [27][28][29][30] have been extensively employed as SAs for demonstrating pulsed laser operations. In particular, TMDs including MoS 2 [18,19,22], MoSe 2 [20][21][22] and WS 2 [22][23][24][25][26] have attracted more attention in the field of ultra-fast optics due to their obvious advantages of a wide absorption range, easy preparation, low cost, fast recovery time, high damage threshold, high third-order nonlinear coefficients, low saturation threshold and suitable bandgap value.…”