The present study examines the extent of academic librarians’ teaching, research, communication, and interpersonal skills; key competencies required for the successful implementation of embedded librarianship in Tanzania. A mixed research approach, integrating both qualitative and quantitative approaches, was deployed to guide the collection of data from 166 librarians and 6 directors. Whereas cross-section survey questionnaires were used to collect data from librarians from six university libraries. Semi-structured face-to-face interviews were used to collect data from directors. Regarding statistical analysis, descriptive statistics were performed to derive frequencies and percentages from quantitative data collected. The qualitative data were analyzed thematically and presented in narrative form. The findings suggest that librarians’ teaching skills and their knowledge of the research cycle are inadequate, while their communication and interpersonal skills are sufficient to allow them to effectively embed their services in their users’ (researchers, students, and teaching staff) activities. To effectively adopt embedded librarianship, the authors recommend the allocation of adequate funds to support diverse external and in-house training, the development of harmonized library and information science (LIS) curriculum, and the use of social media to interact with users.