Ga 1-x Mn x N and Ga 1-x Fe x N thin films and nanostructures were grown by metalorganic chemical vapor deposition. High resolution X-ray diffraction studies demonstrate that the material is high quality single phase similar in quality and lattice parameter to unalloyed GaN. The as-grown epitaxial films exhibit ferromagnetic hysteresis at room temperature as measured by SQUID magnetometry; the strength of the observed volume magnetization is almost an order stronger in similarly grown Mn-doped samples relative to Fe-doped samples. Raman spectroscopy revealed no significant strain introduced by the transition metal incorporation and a low free carrier concentration, and the most prominent additional mode in Mn-doped GaN is attributed to vacancy-related local vibrational modes of the GaN host lattice. A novel growth method has been developed to produce GaN-based nanostructures using a two-step process (GaN deposition followed by an activation step) at low growth temperatures (<850 o C) and V-III ratios (<30). GaMnN nanostructures were grown by introducing Mn to GaN flows under optimal conditions for the formation of nanostructure without the need of an activation step. Manganese icorporation has the tangential benefit that Mn acts as an anti-surfactant, and promotes the low-temperature nucleation of these nanostructures. In addition, experiments have been conducted in which Fe was incorporated into GaN nanostructures at 800 ºC, and room temperature ferromagnetic behavior of GaFeN nanostructures was observed. Atomic force microscopy measurements revealed that Fe, like Mn, affected the surface morphology of the nanostructures by reducing the nanostructure size. These nanostructures showed a systematic variation in coercive field and saturation magnetization with Fe incorporation.