Traditional cooling technologies suffer from several limitations: basically, they all rely on electricity, have high energy needs, and discharge waste heat into the surrounding environment which in turn contributes to global warming and the urban heat island effect. [2][3][4] For these reasons, the recent development of passive radiative sky cooling materials is attracting a growing interest due to its environmentally friendly nature and energy-free working principle. [5] In recent years, hundreds of candidate materials have been proposed, offering a range of passive cooling performances during daytime hours and even under direct sunlight. Two essential requirements for sub-ambient radiative cooling under direct sunlight are a high reflectivity above 90% in the solar spectral range (0.25-2.5 µm), and a strong, preferably selective emissivity in the atmospheric transparency window (8-13 µm). [6,7] This demanding combination of optical properties is generally achieved through both the selection of specific materials with appropriate absorption bands and the micro and nanoengineering of coatings. These materials can be generally divided into four main categories, namely dielectric multilayer films, [8][9][10][11][12] organic-inorganic composite materials, [13][14][15] Coatings for passive radiative cooling applications must be highly reflected in the solar spectrum, and thus can hardly support any coloration without losing their functionality. In this work, a colorful daytime radiative cooling surface based on structural coloration is reported. A designed radiative cooler with a bioinspired array of truncated SiO 2 microcones is manufactured via a self-assembly method and reactive ion etching. Complemented with a silver reflector, the radiative cooler exhibits broadband iridescent coloration due to the scattering induced by the truncated microcone array while maintaining an average reflectance of 95% in the solar spectrum and a high thermal emissivity (ε) of 0.95, owing to the reduced impedance mismatch provided by the patterned surface at infrared wavelengths, reaching an estimated cooling power of ≈143 W m -2 at an ambient temperature of 25 °C and a measured average temperature drop of 7.1 °C under direct sunlight. This strong cooling performance is attributed to its bioinspired surface pattern, which promotes both the aesthetics and cooling capacity of the daytime radiative cooler.