In this paper, three approaches to incorporating nitrogen in CoTiO 3 high-k dielectric films, ion implantation of N 2 + , ion implantation of N + , and N 2 O plasma treatment have been investigated for the new CoTiO 3 high-k dielectrics. All three methods reduced the leakage currents and improved the breakdown characteristics but the N 2 O-plasma treatment produced the best-behaved C-V curves, when compared to the untreated control samples.