Predictor Packing in Developing Unprecedented Shaped Colloidal Particles

Ali, Mubarak; Lin, I-Chun; Yeh, Chia-Shen

doi:10.20944/preprints201801.0039.v4

Cited by 5 publications

(9 citation statements)

References 40 publications

(57 reference statements)

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“…by the splitted electrons [25]. Because of the fixed precursor concentration, the rate of dissociating gold atoms remained the same for a different processing time of solution.…”

Section: Resultsmentioning

confidence: 99%

“…In monolayer assembly, ordering of the atoms is in single layer, they cover region(s) of solution surface by forming the shape more like an arc or a semi-circular shape and at both sides of the center of solution surface (in a standard glass beaker). A layout of the sketch is drawn (in estimation), which is part of another study [25]. particles of that shape where the size of those tiny particles is as per availability of energy per unit atom (area) [18].…”

Section: Resultsmentioning

confidence: 99%

“…Electrons of the atoms introducing the diffusion mechanism is as per their pulling or [25]. For the case of one-dimensional shape of the particles, atoms of triangular-shaped tiny particles elongated less, thus, developing more width in each structure of smooth element [31]; in the case of packing of tiny-shaped particles (to develop them) in shapelike triangular or hexagonal, a similar mechanism is involved, as for the case of developing rod-or bar-shaped particles but their arrival to pack at centre of light glow is from the different zones of the solution surface.…”

Section: Resultsmentioning

confidence: 99%

“…However, the put-forth explanation may be re-visited upto a certain extent when some other amount of precursor concentration is utilized along with different processing unit. Increasing the process time under optimized precursor concentration for fixed amount results into develop the maximum number of triangular-shaped tiny particles[25].In the packing of tiny-sized particles while developing different extended shapes of particles, adjacent-orientation of electrons in their atoms is not appeared to work uniformly and their tiny-sized particles didn't develop in an equilateral triangular-shape.Instead of perfect packing of such tiny-sized particles, due to geometric constraint, they pack under mixed-behavior of exerting forces, which results into their misfit packing, thus, leaving the afterward packing regions in irregular manner where packing of tinysized particles developing a particle deals a further non-uniformity. As shown in the particles developed at the shortest process duration, large tiny-sized particles with an average size bigger than 20 nm deal unfit boundary to maintain packing with respect to the center of developing particle.…”

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Formation of tiny particles and their extended shapes: origin of physics and chemistry of materials

2019

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Tiny-sized particles under the scheme of monolayer assembly, comprising gold atoms, developed at a different processing time in a pulse-based process. For a different processing time, atoms bind into different tiny particles under the placing packets of nanoshape energy where they elongate as per arrangement and when in one-dimensional arrays, they convert into structures of smooth elements. For different processing time and where tiny particles possess triangular-shape, they pack to develop extended shapes where development rate of an anisotropic particle is not more than millisecond time. Increasing the processing time of solution upto certain duration increases the number of developing tiny particles in a triangular-shape, so, their extended shapes also. Uniformly adjacent-orientation of electrons in atoms of tinyshaped particle is because of exerting uniform surface force along their opposite poles as per gained potential energy where stretching of their clamped energy knots is remained orientational-based. At a different processing time, inter-spacing distance of spotted intensity spots in selective area photons reflection patterns of particles is remained the same as for the case of their structures of smooth elements visualized through transmission microscope high-resolution images. When the forceful coinciding of two parallel structures of smooth elements is occurred, they bind into single element structure (of smooth element) by a bit overlying inner sides, thus, giving its double width where certain filled state electrons and unfilled energy knots (belonging to sides of elongated atoms of parallel structures of smooth elements) coordinate to adhere. This 2 study discusses the formation of tiny particles following by their extended shapes at different processing time of gold solution while employing a pulse-based electronphoton solution-interface process where they become the origin of physics and chemistry of materials by discussing many commonly-known phenomena and processes, so, opening the alternative routes to design materials and explore science.

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“…by the splitted electrons [25]. Because of the fixed precursor concentration, the rate of dissociating gold atoms remained the same for a different processing time of solution.…”

Section: Resultsmentioning

confidence: 99%

Section: Resultsmentioning

confidence: 99%

Section: Resultsmentioning

confidence: 99%

mentioning

confidence: 99%

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Formation of tiny particles and their extended shapes: origin of physics and chemistry of materials

2019

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“…A detail on the formation of triangular-shaped tiny particle along with elongation of atoms is given elsewhere [40]. Gold particles of unprecedented shapes developed under tailored process parameters as discussed elsewhere [41]. Different binding mechanisms in evolving structures of solid atoms having different-dimension and different-format have been discussed elsewhere [42] where conservation forces involved to transform heat energy into binding energy under confined inter-state electron-dynamics.…”

Section: Resultsmentioning

confidence: 99%

Tapping Opportunity of Tiny-Shaped Particles and Role of Precursor in Developing Shaped Particles

Ali

Lin

Yeh

2018

NANO

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113

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Metallic colloids are frequently used in industry and provide understanding of science at microns to nanometers scales along with their applicability for various technologically important applications. Present investigations deal morphology-structure of gold, silver and their binary composition while processing the certain amount of their solutions in a newly designed process and tap opportunities of developing tiny shaped particles. At tuned ratio of pulse OFF to ON time and when gold solution was processed, several tiny shaped particles developed at solution surface. Such tiny particles deal force at the tip of each converted structure of smooth element under the steady-state immersing behavior pointing toward common centre to pack for developing different geometric anisotropic shaped particles. Under identical parameters along with pulse time, processing solutions of silver nitrate and binary composition of chloroauric acid-silver nitrate result into develop tiny particles having no specific shape where their packing deal mixed behavior of force resulting into develop distorted particles.Elongation and deformation of gold and silver atoms while in different structures is because of the plastically-driven behavior of electrons as per stretching of their clamped energy knots. In structure of three-dimensional where electrons of atoms do not deal transition require for elongation they retain the structure as it is known in hcp structure or two-dimensional structure. Different nature of precursors along with morphologystructure of particles is discussed in this paper opening abundant avenues of research.

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RETRACTED ARTICLE: The effect of the electronic structure, phase transition, and localized dynamics of atoms in the formation of tiny particles of gold

Ali

Lin

2017

J Nanopart Res

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In addition to the self-governing properties, tiny-sized particles of metallic colloids are the building blocks of large-sized particles. Thus, their study has been the subject of many studies. A tiny-sized particle developed at or inside the solution depends on the attained-dynamics of atoms where different mechanisms of their bindings occur. When a protocol energy is supplied to transitional-state atoms of monolayer assembly, it binds them in own shape. Atoms of one-dimensional arrays elongate uniformly under force-exertion to electrons along opposite poles to form structures of smooth elements of tiny particles. At solution surface, impinging electron streams at a fixed angle results into elongate further the already elongated atoms of structures of smooth elements through gained forced energy of carried photons. Travelling photons of different forcing energies along air-solution interface further shape structures of smooth elements. Inside the solution or near to interface, gold atoms also form tiny particles of different shape-structure where, in addition to their attained-dynamics, miscellaneous factors contribute as well. Again, suitably amalgamated gold atoms when in the neutral state, they execute confined inter-state electron-dynamics to self-generate bind energy where they are not required to be uplifted at solution surface for binding under protocol energy. Tiny-sized particles evolve structures in the original format instead of developing structures if localized dynamics of atoms favor execution of electron-dynamics where they do not require nano-energy to design structures. This study highlights the fundamental process of 2 formation of different tiny particles where electronic structure, phase transition and localized dynamics of gold atoms influence. Such a tool of processing materials opens several possibilities to develop engineered materials of specific properties.

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Predictor Packing in Developing Unprecedented Shaped Colloidal Particles

Cited by 5 publications

References 40 publications

Formation of tiny particles and their extended shapes: origin of physics and chemistry of materials

Formation of tiny particles and their extended shapes: origin of physics and chemistry of materials

Tapping Opportunity of Tiny-Shaped Particles and Role of Precursor in Developing Shaped Particles

RETRACTED ARTICLE: The effect of the electronic structure, phase transition, and localized dynamics of atoms in the formation of tiny particles of gold

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