“…In order to satisfy the utilization requirements of this compound in recording media, permanent magnets, microwave devices and magneto-optics, etc. [6][7][8], many studies have focused on tailoring hexaferrites with modified magnetic properties by substituting Fe 3+ ions with divalent, trivalent and tetravalent cations or cations combinations [9][10][11][12][13][14][15][16][17][18]. For this purpose, several methods have been used to prepare hexaferrite particles including sol-gel method [19,20], mechano-combusition method [21], microwave-induced hydrothermal reaction [22], ammonium nitrate melt technique [23], reverse micelle technique [24], citrate-nitrate gel combustion method [25], co-precipitation method [26] and ball milling method [27,28].…”