A double-low-temperature-buffer variable-temperature growth scheme was studied for fabrication of strain-relaxed thin Si 0.6 Ge 0.4 layer on Si͑001͒ by using molecular beam epitaxy ͑MBE͒, with particular focuses on the influence of growth temperature of individual low-temperature-buffer layers on the relaxation process and final structural qualities. The low-temperature buffers consisted of a 40 nm Si layer grown at an optimized temperature of ϳ400°C, followed by a 20 nm Si 0.6 Ge 0.4 layer grown at temperatures ranging from 50 to 550°C. A significant relaxation increase together with a surface roughness decrease both by a factor of ϳ2, accompanied with the cross-hatch/ cross-hatch-free surface morphology transition, took place for the sample containing a low-temperature Si 0.6 Ge 0.4 layer that was grown at ϳ200°C. This dramatic change was explained by the association with a certain onset stage of the ordered/disordered growth transition during the low-temperature MBE, where the high density of misfit dislocation segments generated near surface cusps largely facilitated the strain relaxation of the top Si 0.6 Ge 0.4 layer.