2013
DOI: 10.1002/adom.201300385
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Second Harmonic Generation Circular Dichroism from Self‐Ordered Hybrid Plasmonic–Photonic Nanosurfaces

Abstract: Hybrid structures composed by self-ordered dielectric nanospheres and partially covered by gold nanocrescents, produce efficient second harmonic generation signals due to the cooperative effect of localized plasmon excitation and 2D Bragg gratings. Asymmetries in the geometric shape of the gold nanocrescents induce a circularly polarized optical response

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Cited by 51 publications
(48 citation statements)
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“…In addition to 3D photonic crystals, 2D colloidal monolayers can also be tuned to create many different optical materials and properties. For example, the monolayer can be used for shadow deposition to generate different shapes of deposited materials, 97,120,124,186 used as an etch mask to generate high aspect ratio structures with high order, 166,187,188 inverted/textured to create antireflective coatings for reducing the amount of reflected light from a substrate surface, 95 or deformed to generate structurally colored patterns on a substrate. 112 Interesting coupling effects can be observed between the photonic modes of an opal and the plasmonic modes of thin metals deposited on top of the crystal.…”
Section: Factors Affecting Optical Applicationsmentioning
confidence: 99%
See 1 more Smart Citation
“…In addition to 3D photonic crystals, 2D colloidal monolayers can also be tuned to create many different optical materials and properties. For example, the monolayer can be used for shadow deposition to generate different shapes of deposited materials, 97,120,124,186 used as an etch mask to generate high aspect ratio structures with high order, 166,187,188 inverted/textured to create antireflective coatings for reducing the amount of reflected light from a substrate surface, 95 or deformed to generate structurally colored patterns on a substrate. 112 Interesting coupling effects can be observed between the photonic modes of an opal and the plasmonic modes of thin metals deposited on top of the crystal.…”
Section: Factors Affecting Optical Applicationsmentioning
confidence: 99%
“…112 Interesting coupling effects can be observed between the photonic modes of an opal and the plasmonic modes of thin metals deposited on top of the crystal. [189][190][191][192][193] Colloids can also be used for antireflective coating applications. 85 In particular, colloidal monolayers have been used to create porous, graded-index materials with low reflectivity by, for example, plasma etching of colloidal monolayers, 194 inverting the monolayer, 95 or using the monolayer as an etching mask to generate pillars.…”
Section: Factors Affecting Optical Applicationsmentioning
confidence: 99%
“…5,14 In Fig. In order to investigate the symmetry breaking induced by the geometry, we measured the SHG signal generated by generally elliptical polarized pulsed light.…”
Section: Samples and Nonlinear Optical Measurementsmentioning
confidence: 99%
“…Enhancement of the optical electric field stronger than that due to the LSP alone was reported. Au nanoparticles/nanostructure were used to exhibit the LSP resonance by some studies 4,6 because of the chemical stability of Au. Thus, robustness in applications is expected.…”
Section: Introductionmentioning
confidence: 99%
“…On the other hand, Ag nanoparticles/nanostructure were employed in some studies 1, 2, 5, 3 because of their high performance of the electric field enhancement. For the photonic crystal material, polystyrene (a regular array of particles or a regular pattern) was selected in some studies, 2,4,3,6 while poly(methyl methacrylate) was used by Xu et al 5 and silica was used by Kim et al 1 An advantage of polystyrene is narrow particle size dispersity. Polystyrene suspensions with the dispersity less than few percent in the coefficient of variation can be synthesized by a soap-free emulsion polymerization.…”
Section: Introductionmentioning
confidence: 99%