The intensity of natural disasters has increased recently, causing buildings' damages which need to be reinforced to prevent their destruction. To improve the seismic proofing capability of Accumulated Semiactive Hydraulic Damper, it is converted to an Active Interaction Control device and synchronous control and predictive control methods are proposed. The full-scale shaking table test is used to test and verify the seismic proofing capability of the proposed AIC with these control methods. This study examines the shock absorption of test structure under excitation by external forces, influences of prediction time, stiffness of the auxiliary structure, synchronous switching, and asynchronous switching on the control effects, and the influence of control locations of test structure on the control effects of the proposed AIC. Test results show that, for the proposed AIC with synchronous control and predictive control of 0.10∼0.13 seconds, the displacement reduction ratios are greater than 71%, the average acceleration reduction ratios are, respectively, 36.2% and 36.9%, at the 1st and 2nd floors, and the average base shear reduction ratio is 29.6%. The proposed AIC with suitable stiffeners for the auxiliary structure at each floor with synchronous control and predictive control provide high reliability and practicability for seismic proofing of buildings.