2011
DOI: 10.1007/s12274-011-0155-4
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Spatially resolved photoelectric performance of axial GaAs nanowire pn-diodes

Abstract: The spatially resolved photoelectric response of a single axial GaAs nanowire pn-diode has been investigated with scanning photocurrent and Kelvin probe force microscopy. Optical generation of carriers at the pn-junction has been shown to dominate the photoresponse. A photocurrent of 88 pA, an open circuit voltage of 0.56 V and a fill factor of 69% were obtained under AM 1.5 G conditions. The photocurrent followed the increasing photoexcitation with 0.24 A/W up to an illumination density of at least 90 W/cm 2 … Show more

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Cited by 32 publications
(36 citation statements)
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“…From the literature, one can find the electron mobility (µ) of GaAs NW around 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60 9 4000 cm 2 V -1 s -1 and electron lifetime (τ) in the order of 10 2 ps, [29][30][31][32][33] resulting in an electron diffusion length around 1 µm as estimated by equation (µτkT/e) 1/2 (where kT/e is constant), that is in a good agreement with the electron beam induced current (EBIC) and Kelvin probe force microscopy (KPFM) measurements. 34,35 All these are completely consistent with our results presented in Figure 2d, in which the photovoltaic performance statistics (based on 100 single NW devices) explicitly show that the high efficiency and large J SC are only obtained for the channel length <1 µm. The channel length dependent V OC and FF are given in Supporting Information Figure S3.…”
Section: Resultssupporting
confidence: 90%
“…From the literature, one can find the electron mobility (µ) of GaAs NW around 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 51 52 53 54 55 56 57 58 59 60 9 4000 cm 2 V -1 s -1 and electron lifetime (τ) in the order of 10 2 ps, [29][30][31][32][33] resulting in an electron diffusion length around 1 µm as estimated by equation (µτkT/e) 1/2 (where kT/e is constant), that is in a good agreement with the electron beam induced current (EBIC) and Kelvin probe force microscopy (KPFM) measurements. 34,35 All these are completely consistent with our results presented in Figure 2d, in which the photovoltaic performance statistics (based on 100 single NW devices) explicitly show that the high efficiency and large J SC are only obtained for the channel length <1 µm. The channel length dependent V OC and FF are given in Supporting Information Figure S3.…”
Section: Resultssupporting
confidence: 90%
“…This study represents an important advance in fabricating core-shell heterojunction NWs for high-performance optoelectronic applications [29]. Wang et al developed an efficient and highly sensitive broad band UV/VIS photodetector based on wide band gap ZnO/ZnS heterojunction 3D core/shell nanowire array [37]. The abrupt interface between ZnO and ZnS plays a dominant role in photon absorption via an indirect type-II transition which was strongly manifested in the photodetection of visible illumination (blue and green).…”
Section: Photodetectorsmentioning
confidence: 97%
“…In addition, 1-D axial heterojunction is considered to be fabricated more easily than core-shell approaches and expected to exhibit lower leakage currents and, therefore, should possess a superior rectifying behavior compared to radial structures [37]. 1-D axial heterojunctions, based on II-VI compound semiconductor nanostructures, have also caught the eye of investigators and present excellent performance.…”
Section: -D Axial Heterojunctionsmentioning
confidence: 99%
“…However, using a simple analysis with a projected absorption area equal to the i-region, we achieve similar efficiencies as previously published single-NW devices. 6,30 We plotted the short-circuit current vs. laser power (Fig. 2(b)) and found a linear dependence over five orders of magnitude.…”
mentioning
confidence: 95%
“…4) and GaAs (Ref. 30) devices. The rectifying behavior demonstrates that HCl prevents the overgrowth of a conductive n-type shell.…”
mentioning
confidence: 99%