Abstract. With the rising anthropogenic emissions from human activities, elevated
concentrations of air pollutants have been detected in the hemispheric air
flows in recent years, aggravating the regional air pollution and deposition
issues. However, the regional contributions of hemispheric air flows to
deposition have been given little attention in the literature. In this light,
we assess the impact of hemispheric transport on sulfur (S) and nitrogen (N)
deposition for six world regions: North America (NA), Europe (EU), South Asia
(SA), East Asia (EA), Middle East (ME) and Russia (RU) in 2010, by using the
multi-model ensemble results from the 2nd phase of the Task Force Hemispheric
Transport of Air Pollution (HTAP II) with 20 % emission perturbation
experiments. About 27 %–58 %, 26 %–46 % and
12 %–23 % of local S, NOx and NH3 emissions and
oxidation products are transported and removed by deposition outside of the
source regions annually, with seasonal variation of 5 % more in winter
and 5 % less in summer. The 20 % emission reduction in the source
regions could affect 1 %–10 % of deposition in foreign continental
regions and 1 %–14 % in foreign coastal regions and the open ocean.
Significant influences are found from NA to the North Atlantic Ocean
(2 %–14 %), and from EA to the North Pacific Ocean
(4 %–10 %) and to western NA (4 %–6 %) (20 % emission
reduction). The impact on deposition caused by short-distance transport
between neighboring regions (i.e., from EU to RU) occurs throughout the whole
year (slightly stronger in winter), while the long-range transport (i.e.,
from EA to NA) mainly takes place in spring and fall, which is consistent
with the seasonality found for hemispheric transport of air pollutants.
Deposition in the emission-intensive regions such as US, SA and EA is
dominated (∼80 %) by own-region emissions, while deposition in the
low-emission-intensity regions such as RU is almost equally affected by
foreign exported emissions (40 %–60 %) and own-region emissions. We
also find that deposition of the coastal regions or the near-coastal open
ocean is twice more sensitive to hemispheric transport than the non-coastal
continental regions, especially for regions in the downwind direction of
emission sources (i.e., west coast of NA). This study highlights the
significant impacts of hemispheric transport of air pollution on the
deposition in coastal regions, the open ocean and low-emission-intensity
regions. Further research is proposed to improve the ecosystem and human
health, with regards to the enhanced hemispheric air flows.