Infrared laser-absorption spectroscopy (IR-LAS) sensors play an important role in diagnosing and characterizing a wide range of combustion systems. Of all the laser-diagnostic techniques, LAS is arguably the most versatile and quantitative, as it has been used extensively to provide quantitative, species-specific measurements of gas temperature, pressure, composition and velocity in both laboratory-and industrial-scale systems. Historically, most IR-LAS work has been conducted using tunable diode lasers, however, today's researchers have access to a wide range of light sources that provide unique sensing capabilities and convenient access to nearly the entire IR spectrum (≈1 to 20 μm). In particular, the advent of room-temperature wavelength-tunable mid-infrared semiconductor lasers (e.g., interband-and quantum-cascade lasers) and hyperspectral light sources (e.g., Fourierdomain mode-locked lasers, dispersed supercontinuum lasers, and frequency combs) has provided a number of unique capabilities that combustion researchers have exploited. The primary goal of this review paper is to document the recent development, application, and current capabilities of IR-LAS sensors for laboratory-and industrial-scale combustors and propulsion systems. A thorough review and description of the fundamental spectroscopy governing the accuracy of such sensors, and recent findings and databases that enable improved modeling of molecular absorption spectra will be provided. Modern light sources and the most commonly used diagnostic techniques are also discussed.