Aluminum dross, as a hazardous waste product, causes harm to the environment and humans, since the AlN it contains chemically reacts with water to produce ammonia. In the present study, a formula for modifying the AlN content in aluminum dross is proposed for the first time, by investigating the components of aluminum dross and changes in their respective contents during the hydrolysis process. Meanwhile, the effects of such hydrolysis parameters as time, temperature, and rotational speed on the hydrolysis rate of aluminum dross are explored. Furthermore, regression analysis is performed on the hydrolysis parameters and objective functions. The results show that as the reaction time increases, the variation in AlN content in aluminum dross decelerates gradually after modification. The hydrolysis rate is the fastest in the initial 4 h, which essentially stagnates after 20 h. The rise in temperature can significantly accelerate the AlN hydrolysis in aluminum dross, while the rotational speed has a non-obvious effect on the hydrolysis rate of AlN in aluminum dross. Regression analysis and secondary simplification are performed on the hydrolysis parameters and the modified AlN content, revealing that the relative error between the theoretical and experimental values is ≤ ±9.34%. The findings of this study have certain guiding significance for predicting and controlling modified AlN content in aluminum dross during hydrolysis.