We describe and show results from a series of field campaigns that used balloonborne instruments launched from India and Saudi Arabia during the summers 2014–17 to study the nature, formation, and impacts of the Asian Tropopause Aerosol Layer (ATAL). The campaign goals were to i) characterize the optical, physical, and chemical properties of the ATAL; ii) assess its impacts on water vapor and ozone; and iii) understand the role of convection in its formation. To address these objectives, we launched 68 balloons from four locations, one in Saudi Arabia and three in India, with payload weights ranging from 1.5 to 50 kg. We measured meteorological parameters; ozone; water vapor; and aerosol backscatter, concentration, volatility, and composition in the upper troposphere and lower stratosphere (UTLS) region. We found peaks in aerosol concentrations of up to 25 cm–3 for radii > 94 nm, associated with a scattering ratio at 940 nm of ∼1.9 near the cold-point tropopause. During medium-duration balloon flights near the tropopause, we collected aerosols and found, after offline ion chromatography analysis, the dominant presence of nitrate ions with a concentration of about 100 ng m–3. Deep convection was found to influence aerosol loadings 1 km above the cold-point tropopause. The Balloon Measurements of the Asian Tropopause Aerosol Layer (BATAL) project will continue for the next 3–4 years, and the results gathered will be used to formulate a future National Aeronautics and Space Administration–Indian Space Research Organisation (NASA–ISRO) airborne campaign with NASA high-altitude aircraft.
Abstract. To date, several satellites measurements are available which can provide profiles of temperature and water vapour with reasonable accuracies. However, the temporal resolution has remained poor, particularly over the tropics, as most of them are polar orbiting. At this juncture, the launch of INSAT-3D (Indian National Satellite System) by the Indian Space Research Organization (ISRO) on 26 July 2013 carrying a multi-spectral imager covering visible to longwave infrared made it possible to obtain profiles of temperature and water vapour over India with higher temporal and vertical resolutions and altitude coverage, besides other parameters. The initial validation of INSAT-3D data is made with the high temporal (3 h) resolution radiosonde observations launched over Gadanki (13.5 • N, 79.2 • E) during a special campaign and routine evening soundings obtained at 12:00 UTC (17:30 LT). We also compared INSAT-3D data with the radiosonde observations obtained from 34 India Meteorological Department stations. Comparisons were also made over India with data from other satellites like AIRS, MLS and SAPHIR and from ERA-Interim and NCEP reanalysis data sets. INSAT-3D is able to show better coverage over India with high spatial and temporal resolutions as expected. Good correlation in temperature between INSAT-3D and in situ measurements is noticed except in the upper tropospheric and lower stratospheric regions (positive bias of 2-3 K). There is a mean dry bias of 20-30 % in the water vapour mixing ratio. Similar biases are noticed when compared to other satellites and reanalysis data sets. INSAT-3D shows a large positive bias in temperature above 25 • N in the lower troposphere. Thus, caution is advised when using these data for tropospheric studies. Finally it is concluded that temperature data from INSAT-3D are of high quality and can be directly assimilated for better forecasts over India.
Despite being rare, large volcanic eruptions can have a long-lasting impact on the chemistry, radiation, and dynamics of the stratosphere. This study attempts to quantify the changes in the stratospheric water vapour and its relationship to temperature and ozone observed from space-based Microwave Limb Sounder (MLS) observations during the submarine volcano eruption Hunga Tonga-Hunga Ha’apai that occurred on 15 January 2022. The most notable aspect of this eruption is the plumes, which are water vapour columns that reached higher altitudes (1 hPa (47.6 km)) than earlier eruptions. We discovered that the eruption injected a record amount of water vapour (6–8 ppmv) directly into the stratosphere from 38–10 hPa vertically, which is present even after one year. The majority of water vapour is confined to the Southern Hemisphere (SH) tropics, i.e., 30°S to 5°N, and gradually descends to the SH polar latitudes over time. The WV from the lower stratosphere reaches mesospheric altitudes during January 2023. We quantify the impact of increased water vapour on temperature and ozone as well. Temperatures begin to fall during the month of March in the regions where there is an increase in water vapour. A ~5 K cooling occurs in July and August as a result of the thermal adjustment to the extra water vapour IR cooling. Our analysis shows a decrease in ozone caused by an increase in water vapour. Significant variability is observed in all three parameters at 26 km compared to other levels. Further, we noticed that after one year of eruption, the water vapour, Temperature and Ozone did not reach the background values. It is possible that this unusual eruption produced a different atmospheric reaction than other significant volcanic eruptions that have been well investigated.
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