a b s t r a c tRecombination active boron oxygen related defects typically limit the efficiency of solar cells made from boron doped, oxygen rich silicon. This limitation can be overcome by applying a regeneration process that requires slightly elevated temperatures, carrier injection, and the presence of hydrogen in the silicon substrate in order to regenerate quickly and completely.The influence of mid temperature steps up to 400 1C on the regeneration kinetics is investigated and the results can be explained with the efficacy of the regeneration process depending on the hydrogen bonding states prior to regeneration. Boron hydrogen pairs are found to be good candidates to be the relevant hydrogen source during regeneration. The long term stability of the regenerated state is tested under solar cell operating conditions, and the thermal activation energy of its destabilization is determined to be 1.25 70.05 eV.Limiting factors for high speed regeneration processes are discussed, and a high temperature/high illumination procedure is presented, allowing complete regeneration in less than 10 s. This makes regeneration feasible as an in line process in solar cell production.

We demonstrate time-domain sampling of mid-infrared electric field transients and their conjugate counterparts exploiting the dynamical Pockels effect. To this end, the complete polarization change of few-femtosecond probe pulses is studied. An intuitive picture based on a phasor representation is established before gaining quantitative understanding in experiment and theory. In the standard version of electro-optic sampling, the electric field is determined by analyzing the change of ellipticity of the probe polarization. Beyond this, we find that a temporal gradient of the input electric field manifests itself in a rotation of the polarization ellipsoid of the probe. The relative contribution of sum-and difference-frequency mixing processes and their spectral distribution over the near-infrared probe bandwidth are identified as key aspects. If one of these processes dominates, detecting ellipticity changes and polarization rotation as a function of time delay results in two wave forms which are Hilbert transforms of each other. Such conditions may be achieved by angle phase matching in birefringent materials or spectral filtering of the probe after the nonlinear interaction. In this case, a static phase introduced by birefringence or reflection at metallic mirrors results in a specific phase shift of both time traces with respect to the input electric field. Contributions from sum-and difference-frequency generation are found to be equivalent when using electro-optic sensors with isotropic refractive index. Polarization rotations in the lowand high-frequency parts of the probe then tend to cancel out. In this limit, spurious additional phase shifts do not change the phase of the detected transients. This fact leads to a robust recovery of the carrier-envelope phase of the input wave form. Clarifying the role of imperfections of superachromatic phase retarders completes our survey on proper determination of the electric field and its conjugate variable.

Sequences of ultrashort pulses form the basis of extremely precise laser applications ranging from femtosecond spectroscopy, to material microprocessing, to biomedical imaging. Dynamic patterns of temporal solitons—termed “soliton molecules”—inside mode-locked cavities provide yet unexplored means for generating reconfigurable arrangements of ultrashort pulses. Here, we demonstrate the external control of solitonic bound states in widespread erbium-doped fiber lasers via direct electronic modulation of the semiconductor pump source. This straightforward approach allows for switching between discrete soliton doublet states of picosecond separations, employing and relying on laser-intrinsic soliton interactions. We analyze the externally induced dynamics based on real-time switching data acquired by time-stretch dispersive Fourier transform spectroscopy and identify a universal bound-state formation mechanism different from broadly considered models. Owing to the ease of implementation and its intrinsic tunability, our control scheme is readily applicable to various laser platforms enabling, e.g., rapid multipulse measurements and tailored nonlinear light–matter interactions.

Phase-stable electromagnetic pulses in the THz frequency range offer several unique capabilities in timeresolved spectroscopy. However, the diversity of their application is limited by the covered spectral bandwidth. In particular, the upper frequency limit of photoconductive emitters -the most widespread technique in THz spectroscopyreaches only up to 7 THz in regular transmission mode due to the absorption by infrared-active optical phonons. Here, we present ultra-broadband (extending up to 70 THz) THz emission from Au implanted Ge emitter which is compatible with a fibre laser operating at 1.2 and 1.55 m wavelengths at a repetition rates of 10 and 20 MHz, respectively. This opens a perspective for the development of compact THz photonic devices operating up to multi-THz frequencies and compatible with Si CMOS technology.

We explore background-free options to detect mid-infrared (MIR) electric transients. The MIR field and a near-infrared probe interact via sum- (SFG) and difference-frequency generation (DFG) in an electro-optic crystal. An intuitive picture based on a phasor representation and rigorous numerical calculations are used for analysis. It turns out that separating photons generated either by SFG or DFG from the local oscillator via spectral filtering leads to a signal purely proportional the MIR intensity envelope. Background-free phase information may be extracted in a spectral window containing both SFG and DFG components and blocking the local oscillator background based on its orthogonal polarization. This variant leads to signal proportional to the square of the MIR field amplitude. It is limited by the finite efficiency of polarization filtering. The Hilbert transform as a conjugate variable to the electric field in the time domain turns out to play a fundamental role for the context discussed in this paper.