Sequences of ultrashort pulses form the basis of extremely precise laser applications ranging from femtosecond spectroscopy, to material microprocessing, to biomedical imaging. Dynamic patterns of temporal solitons—termed “soliton molecules”—inside mode-locked cavities provide yet unexplored means for generating reconfigurable arrangements of ultrashort pulses. Here, we demonstrate the external control of solitonic bound states in widespread erbium-doped fiber lasers via direct electronic modulation of the semiconductor pump source. This straightforward approach allows for switching between discrete soliton doublet states of picosecond separations, employing and relying on laser-intrinsic soliton interactions. We analyze the externally induced dynamics based on real-time switching data acquired by time-stretch dispersive Fourier transform spectroscopy and identify a universal bound-state formation mechanism different from broadly considered models. Owing to the ease of implementation and its intrinsic tunability, our control scheme is readily applicable to various laser platforms enabling, e.g., rapid multipulse measurements and tailored nonlinear light–matter interactions.

Femtosecond frequency combs are among the most precise measurement tools in existence. They have applications ranging from high-precision spectroscopy and metrology to time-domain quantum physics. Maximizing the passive stability of these instruments is essential to achieve their full potential in fundamental science and high-tech industry. However, the noise mechanisms across the entire operating space of these devices have not been fully characterized. Here the noise properties of fiber-based frequency combs are studied as a function of intracavity dispersion, pump power, and repetition rate. Distinct minima are discovered in this parameter space where the free-running linewidth of the carrier-envelope offset (CEO) frequency f CEO drops below 1 kHz. The individual comb lines are analyzed spread over a wide spectral range producing a complete understanding of the particular contributions to the phase noise and their interplay. Exploiting these findings, combs featuring sharp teeth at specific frequency positions and over the entire spectrum from f CEO to 300 THz are demonstrated. The ultrabroadband stability offered by these compact systems provides a new level of quality for front-end measurement tasks in both time and frequency domains.

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Moth-eye structures are patterned onto gallium selenide surfaces with sub-micrometer precision. In this way, Fresnel reflection losses are suppressed to below one percent within an ultrabroad optical bandwidth from 15 to 65 THz. We tune the geometry by rigorous coupled-wave analysis. Subsequently, ablation with a Ga+ ion beam serves to write optimized structures in areas covering 30 by 30 μm. The benefits are demonstrated via optical rectification of femtosecond laser pulses under tight focusing, resulting in emission of phase-stable transients in the mid-infrared. We analyze the performance of antireflection coating directly in the time domain by ultrabroadband electro-optic sampling.

Measuring an electric field waveform beyond radio frequencies is often accomplished via a second-order nonlinear interaction with a laser pulse shorter than half of the field’s oscillation period. However, synthesizing such a gate pulse is extremely challenging when sampling mid- (MIR) and near- (NIR) infrared transients. Here, we demonstrate an alternative approach: a third-order nonlinear interaction with a relatively long multi-cycle pulse directly retrieves an electric-field transient whose central frequency is 156 THz. A theoretical model, exploring the different nonlinear frequency mixing processes, accurately reproduces our results. Furthermore, we demonstrate a measurement of the real part of a sample’s dielectric function, information that is challenging to retrieve in time-resolved spectroscopy and is therefore often overlooked. Our method paves the way towards experimentally simple MIR-to-NIR time-resolved spectroscopy that simultaneously extracts the spectral amplitude and phase information, an important extension of optical pump-probe spectroscopy of, e.g., molecular vibrations and fundamental excitations in condensed-matter physics.