Cavity quantum electrodynamics (QED) systems allow the study of a variety of fundamental quantum-optics phenomena, such as entanglement, quantum decoherence and the quantum-classical boundary. Such systems also provide test beds for quantum information science. Nearly all strongly coupled cavity QED experiments have used a single atom in a high-quality-factor (high-Q) cavity. Here we report the experimental realization of a strongly coupled system in the solid state: a single quantum dot embedded in the spacer of a nanocavity, showing vacuum-field Rabi splitting exceeding the decoherence linewidths of both the nanocavity and the quantum dot. This requires a small-volume cavity and an atomic-like two-level system. The photonic crystal slab nanocavity--which traps photons when a defect is introduced inside the two-dimensional photonic bandgap by leaving out one or more holes--has both high Q and small modal volume V, as required for strong light-matter interactions. The quantum dot has two discrete energy levels with a transition dipole moment much larger than that of an atom, and it is fixed in the nanocavity during growth.
In this paper we investigate the coherence properties of a quantum dot under two-photon resonant excitation in combination with an additional photo-neutralization laser. The photo-neutralization increases the efficiency of the excitation process and thus, the brightness of the source, by a factor of approximately 1.5 for biexciton-exciton pairs. This enhancement does not degrade the relevant coherences in the system; neither the single photon coherence time, nor the coherence of the excitation process.
We show that resonance fluorescence, i.e. the resonant emission of a coherently driven two-level system, can be realized with a semiconductor quantum dot. The dot is embedded in a planar optical micro-cavity and excited in a wave-guide mode so as to discriminate its emission from residual laser scattering. The transition from the weak to the strong excitation regime is characterized by the emergence of oscillations in the first-order correlation function of the fluorescence, g(τ ), as measured by interferometry. The measurements correspond to a Mollow triplet with a Rabi splitting of up to 13.3 µeV. Second-order-correlation measurements further confirm non-classical light emission. [3,4,5,6,7], as well as photon anti-bunching [8], and were previously only observable in isolated atoms or ions. In addition, QDs can be readily integrated into optical micro-cavities making them attractive for a number of applications, particularly quantum information processing and high efficiency light sources. For example, QDs could be used to realize deterministic solid-state single photon sources [9,10,11] and qubit-photon interfaces [12]. Advances in high-Q cavities have shown that not only can the spontaneous emission rate be dramatically increased by the Purcell effect [13,14], but emission can be reversed in the strong coupling regime [15,16,17]. Despite these efforts, however, quantum dot-based cavity quantum electrodynamics (QED) lacks an ingredient essential to the success of atomic cavity QED, namely the ability to truly resonantly manipulate the two-level system [9,10,11]. Current approaches can at best populate the dot in one of its excited states, which subsequently relaxes in some way to the emitting ground state. This incoherent relaxation has been addressed theoretically [18,19], and experimentally [20] but direct resonant excitation and collection in the ground state has so far not been reported as it is very challenging to differentiate the resonance fluorescence from same-frequency laser scattering off defects, contaminants, etc. In quantum dots without cavities, coherent manipulation of ground-state excitons has nonetheless been achieved with a number of techniques including differential transmission [6], differential * Electronic address: shih@physics.utexas.edu reflectivity [21], four-wave mixing [22], photodiode spectroscopy [7], and Stark-shift modulation absorption spectroscopy [23]. However, none of these is able to collect and use the actual photon emission which limits their use in many potential applications of QDs. This report presents the first measurement of resonance fluorescence in a single self-assembled quantum dot. Described by Mollow in 1969 [24], the resonant emission of a two-state quantum system under strong coherent excitation is distinguished by an oscillatory first-order correlation function, g(τ ), that we observe with interferometry. We use a planar optical micro-cavity to guide the excitation laser between the cavity mirrors and simultaneously enhance the single photon emission in th...
Articles you may be interested inGaAs-based room-temperature continuous-wave 1.59 μ m GaInNAsSb single-quantum-well laser diode grown by molecular-beam epitaxy Appl. Phys. Lett. 87, 231121 (2005); 10.1063/1.2140614Room-temperature, ground-state lasing for red-emitting vertically aligned InAlAs/AlGaAs quantum dots grown on a GaAs(100) substrate Appl.Room-temperature lasing at the wavelength of 1.31 m is achieved from the ground state of an InGaAs/GaAs quantum-dot ensemble. At 79 K, a very low threshold current density of 11.5 A/cm 2 is obtained at a wavelength of 1.23 m. The room-temperature lasing at 1.31 m is obtained with a threshold current density of 270 A/cm 2 using high-reflectivity facet coatings. The temperature-dependent threshold with and without high-reflectivity end mirrors is studied, and ground-state lasing is obtained up to the highest temperature investigated of 324 K.
Data are presented on the influence of p-type modulation doping on the gain characteristics of 1.3 μm InAs quantum dot lasers. The improvement in optical gain leads to very high characteristic temperatures for the lasing threshold that reach 161 K in the temperature range between 0 and 80 °C. 1.3 μm ground state lasing is obtained up to a temperature of 167 °C.
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