We study the transfer of spectral weight in the optical spectra of a strongly correlated electron system as a function of temperature and interaction strength. Within a dynamical mean field theory of the Hubbard model that becomes exact in the limit of large lattice coordination, we predict an anomalous enhancement of spectral weight as a function of temperature in the correlated metallic state and report on experimental measurements which agree with this prediction in V 2 O 3 . We argue that the optical conductivity anomalies in the metal are connected to the proximity to a crossover region in the phase diagram of the model. 71.27.+a, 71.30.+h, 78 Typeset using REVT E X 1
Highly conductive indium zinc oxide prepared by reactive magnetron cosputtering technique using indium and zinc metallic targets J. Vac. Sci. Technol. A 28, 425 (2010); 10.1116/1.3372806 Effects of Zn content on structural and transparent conducting properties of indium-zinc oxide films grown by rf magnetron sputtering High mobility undoped amorphous indium zinc oxide transparent thin films J. Appl. Phys. 98, 073703 (2005); 10.1063/1.2060957 Transparent conducting zinc oxide and indium-tin oxide films prepared by modified reactive planar magnetron sputtering J.
Fundamental energies are determined optically for an ensemble of correlated electrons in an antiferromagnetic insulator, V203. The observed variation of the energy gap and the kinetic energy are compared quantitatively to some approximate solutions of the Hubbard Hamiltonian.PACS numbers: 71.27.+a, 71.30.+h, 78.30.Hv The approach to the metal-insulator transition by a collection of correlated electrons has been a subject of considerable interest since Mott's classic paper [1] We have made measurements with energy resolution less than 1 meV on crystals which we found to be very difficult to anneal, polish, and etch, with the additional difficulty that they crack on passing through the metalinsulator transition that occurs on cooling from room temperature.Based on optical and dc transport characterization of over 10 crystals, we have developed annealing and surface preparation procedures which yield reproducible spectra [17]. We have made reflectivity, R, measurements from the far-infrared to E = 3.5 eV (a frequency, ta, about 27000 crn ') and used the measurements of Shin et al. [18] from 3.5 to 25 eV in our Kramers-Kronig transformations to obtain the optical conductivity, tr.The main part of Fig. 1 [4,5]) which can introduce conducting states into a filled band, and it also differs from disordered doping which primarily introduces impurity states into the gap [1]. We see negligible absorption (except that due to phonons) in the energy gap, and our 0. extrapolated to E = 0 agrees with the (essentially zero) measured dc conductivity, trd"of similarly prepared samples.Qualitatively, the spectra show an energy gap, 2b"with a "soft" edge and a broad peak at higher energy. This
The Rapid Communications section is intended for the accelerated publication of important new results g. ince manuscripts submitted to this section are given priority treatment both in the editorial once and in production, authors sltould explain in their submittal letter why the work justiftes this special handling A. Rapid Communication should be no longer titan 3' printed pages and must be accompanied by an abstract Pa.ge proofs are sent to authors, but, because of the accelerated schedule, publication is not delayed for receipt of corrections unless requested by the author or noted by tile editor
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