The MIX inventory is developed for the years 2008 and 2010 to support the Model Inter-Comparison Study for Asia (MICS-Asia) and the Task Force on Hemispheric Transport of Air Pollution (TF HTAP) by a mosaic of up-to-date regional emission inventories. Emissions are estimated for all major anthropogenic sources in 29 countries and regions in Asia. We conducted detailed comparisons of different regional emission inventories and incorporated the best available ones for each region into the mosaic inventory at a uniform spatial and temporal resolution. Emissions are aggregated to five anthropogenic sectors: power, industry, residential, transportation, and agriculture. We estimate the total Asian emissions of 10 species in 2010 as follows: 51.3 Tg SO2, 52.1 Tg NOx, 336.6 Tg CO, 67.0 Tg NMVOC (non-methane volatile organic compounds), 28.8 Tg NH3, 31.7 Tg PM10, 22.7 Tg PM2.5, 3.5 Tg BC, 8.3 Tg OC, and 17.3 Pg CO2. Emissions from China and India dominate the emissions of Asia for most of the species. We also estimated Asian emissions in 2006 using the same methodology of MIX. The relative change rates of Asian emissions for the period of 2006–2010 are estimated as follows: −8.1 % for SO2, +19.2 % for NOx, +3.9 % for CO, +15.5 % for NMVOC, +1.7 % for NH3, −3.4 % for PM10, −1.6 % for PM2.5, +5.5 % for BC, +1.8 % for OC, and +19.9 % for CO2. Model-ready speciated NMVOC emissions for SAPRC-99 and CB05 mechanisms were developed following a profile-assignment approach. Monthly gridded emissions at a spatial resolution of 0.25° × 0.25° are developed and can be accessed from http://www.meicmodel.org/dataset-mix
<p><strong>Abstract.</strong> To tackle the problem of severe air pollution, China has implemented active clean air policies in recent years. As a consequence, the emissions of major air pollutants have decreased and the air quality has substantially improved. Here, we quantified China's anthropogenic emission trends from 2010&#8211;2017 and identified the major driving forces of these trends by using a combination of bottom-up emission inventory and Index Decomposition Analysis (IDA) approaches. The relative change rates of China's anthropogenic emissions during 2010&#8211;2017 are estimated as follows: &#8722;62&#8201;% for SO<sub>2</sub>, &#8722;17&#8201;% for NO<sub>x</sub>, +11&#8201;% for NMVOC, +1&#8201;% for NH<sub>3</sub>, &#8722;27&#8201;% for CO, &#8722;38&#8201;% for PM<sub>10</sub>, &#8722;35&#8201;% for PM<sub>2.5</sub>, &#8722;27&#8201;% for BC, &#8722;35&#8201;% for OC, and +18&#8201;% for CO<sub>2</sub>. The IDA results suggest that emission control measures are the main drivers of this reduction, in which the pollution controls on power plants and industries are the most effective mitigation measures. The emission reduction rates markedly accelerated after the year 2013, confirming the effectiveness of China's Clean Air Action that was implemented in 2013. We estimated that during 2013&#8211;2017, China's anthropogenic emissions decreased by 59&#8201;% for SO<sub>2</sub>, 21&#8201;% for NO<sub>x</sub>, 23&#8201;% for CO, 36&#8201;% for PM<sub>10</sub>, 33&#8201;% for PM<sub>2.5</sub>, 28&#8201;% for BC, and 32&#8201;% for OC. NMVOC emissions increased by 11&#8201;% and NH<sub>3</sub> emissions remained stable from 2010&#8211;2017, representing the absence of effective mitigation measures for NMVOC and NH<sub>3</sub> in current policies. The relative contributions of different sectors to emissions have significantly changed after several years' implementation of clean air policies, indicating that it is paramount to introduce new policies to enable further emission reductions in the future.</p>
This paper, which focuses on emissions from China's coal-fired power plants during 1990-2010, is the second in a series of papers that aims to develop a highresolution emission inventory for China. This is the first time that emissions from China's coal-fired power plants were estimated at unit level for a 20-year period. This inventory is constructed from a unit-based database compiled in this study, named the China coal-fired Power plant Emissions Database (CPED), which includes detailed information on the technologies, activity data, operation situation, emission factors, and locations of individual units and supplements with aggregated data where unit-based information is not available. Between 1990 and 2010, compared to a 479 % growth in coal consumption, emissions from China's coal-fired power plants increased by 56, 335, and 442 % for SO 2 , NO x , and CO 2 , respectively, and decreased by 23 and 27 % for PM 2.5 and PM 10 respectively. Driven by the accelerated economic growth, large power plants were constructed throughout the country after 2000, resulting in a dramatic growth in emissions. The growth trend of emissions has been effectively curbed since 2005 due to strengthened emission control measures including the installation of flue gas desulfurization (FGD) systems and the optimization of the generation fleet mix by promoting large units and decommissioning small ones. Compared to previous emission inventories, CPED significantly improved the spatial resolution and temporal profile of the power plant emission inventory in China by extensive use of underlying data at unit level. The new inventory developed in this study will enable a close exami-nation of temporal and spatial variations of power plant emissions in China and will help to improve the performances of chemical transport models by providing more accurate emission data.
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