Non-equilibrium atmospheric-pressure plasmas have recently become a topical area of research owing to their diverse applications in health care and medicine, environmental remediation and pollution control, materials processing, electrochemistry, nanotechnology and other fields. This review focuses on the reactive electrons and ionic, atomic, molecular, and radical species that are produced in these plasmas and then transported from the point of generation to the point of interaction with the material, medium, living cells or tissues being processed. The most important mechanisms of generation and transport of the key species in the plasmas of atmospheric-pressure plasma jets and other non-equilibrium atmosphericpressure plasmas are introduced and examined from the viewpoint of their applications in plasma hygiene and medicine and other relevant fields. Sophisticated high-precision, timeresolved plasma diagnostics approaches and techniques are presented and their applications to monitor the reactive species and plasma dynamics in the plasma jets and other discharges, both in the gas phase and during the plasma interaction with liquid media, are critically reviewed. The large amount of experimental data is supported by the theoretical models of reactive species generation and transport in the plasmas, surrounding gaseous environments, and plasma interaction with liquid media. These models are presented and their limitations are discussed. Special attention is paid to biological effects of the plasma-generated reactive oxygen and nitrogen (and some other) species in basic biological processes such as cell metabolism, proliferation, survival, etc. as well as plasma applications in bacterial inactivation, wound healing, cancer treatment and some others. Challenges and opportunities for theoretical and experimental research are discussed and the authors' vision for the emerging convergence trends across several disciplines and application domains are presented to stimulate critical discussions and collaborations in the future. 4 3.5 Optical absorption spectroscopy 3.5.1 Ozone 3.5.2 UV broadband absorption of OH density 3.5.3 Cavity ring-down spectroscopy 3.5 Selected non-optical techniques 3.5.1 Mass spectrometry 3.5.2 Flow visualization 3.5.3 Electron paramagnetic resonance spectroscopy 4. Temporal and spatial behaviour of key reactive species 4.1 Electron density (n e) 4.2 O atoms 4.2.1 Effect of admixture of O 2 /air on O concentration 4.2.2 Diffusion effect of shielding gas on O production 4.3 OH radical 4.3.1 Effect of H 2 O admixture on OH concentration 4.3.2 Effect of gas flow on OH concentration 4.3.3 Effect of O 2 on OH production 4.3.4 Effect of the treated samples on OH concentration 4.3.4.1 Effect of humidity of treatment sample on OH distribution 4.3.4.2 Effect of sample conductivity on OH distribution 4.3.4.3. Effect of the amplitude of the applied voltage on OH distribution 4.3.4.4. The effect of gas flow on OH distribution 4.3.4.5. The effect of the surface characteristics on OH distribution 4.3.5 Effe...

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The results of simulation of positive streamer propagation along a helium jet in ambient air are presented. A two-dimensional axially symmetric streamer model, accounting for variation of helium–air mixture composition in the jet, is used. The obtained distributions of plasma parameters have a ring-shaped structure, typical for plasma bullets. The calculated radial profiles of emitting nitrogen molecules agree with experimental data.

The paper discusses the relation between streamer velocity and diameter that follows from an analytical approach to description of the streamer head structure. It is shown that using measured data for streamer velocity and diameter one can evaluate the electric field in the streamer head. The analytical approach predicts that for positive streamers a minimum diameter exists, inversely proportional to the gas density.

The results of two-dimensional (2D) numerical simulation of single positive streamer development in atmospheric air in sphere - plane electrode configuration are presented. Correlation of streamer parameters with sphere radius and applied voltage U is revealed. The values of the electric field at the streamer head and in the channel are shown to be almost independent of and U and equal to 150 - 180 and correspondingly. Streamer velocity and radial dimensions linearly increase with U, the coefficient in these linear relations being independent of . Comparison of the results obtained by 2D modelling and in the frame of the commonly used 1D (or quasi-2D) models is made.