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This paper firstly reports key factors which are to be necessarily considered for the successful two-bit (four-level) cell operation in a phase-change random access memory (PRAM). They are 1) the writeand-verify (WAV) writing of four-level resistance states and 2) the moderate-quenched (MQ) writing of intermediate resistance levels, 3) the optimization of temporal resistance increase (so-called resistance drift) and 4) of resistance increase after thermal annealing. With taking into account of them, we realized a two-bit cell operation in diodeswitch phase change memory cells with 90nm technology. All of four resistance levels are highly write endurable and immune to write disturbance above 10 8 cycles, respectively. In addition, they are nondestructively readable above 10 7 read pulses at 100ns and 1uA. IntroductionPhase-change random access memory (PRAM) is most promising to realize a multi-level cell (MLC) operation because it has very wide range of resistance across two orders of magnitude or the higher, with respect to writing current. According to the PRAM road map [1], it is expected that highest memory densities of PRAM become comparable to conventional memories such as NOR Flash and DRAM in coming years when MLC operation is fully accomplished. In this paper, we systematically investigated a four-level (two-bit) cell operation in diode-switch phase change memory cells with 90nm technology and discussed its possibilities and issues as well.

Silicone-acrylic resins were synthesized to prepare superweatherable paints for building materials. The raw materials used were n-butyl acrylate, methyl methacrylate, and n-butyl methacrylate as acrylic monomers and 3-methacryloxypropyltrimethoxysilane (MPTS) as a silicone monomer reactive with the acrylic monomers. Acrylic copolymers were synthesized such that their glass-transition temperatures were adjusted to 30°C and their MPTS contents were varied to 10, 20, and 30 wt %. As the content of silicone and MPTS increased, average molecular weight and viscosity increased, and thermal stability at high temperatures improved. When we tested the properties of coatings by blending the synthesized silicone-acrylic resins with a white pigment, adhesion was superior with various substrates, and their properties were suitable on the whole. Weatherability was tested by an outdoor exposure test with a weather-ometer and an accelerated weathering tester, and their results showed that silicone-acrylic resin composed of 30 wt % MPTS was a superweatherable coating.

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