The strain distribution in heterostructured wurtzite InAs/InP nanowires is measured by a peak finding technique using high resolution transmission electron microscopy images. We find that nanowires with a diameter of about 20 nm show a 10 nm strained area over the InAs/InP interface and the rest of the wire has a relaxed lattice structure. The lattice parameters and elastic properties for the wurtzite structure of InAs and InP are calculated and a nanowire interface is simulated using finite element calculations. Both the method and the experimental results are validated using a combination of finite element calculations and image simulations.
We report tunneling spectroscopy measurements of the Zeeman spin splitting in InAs few-electron quantum dots. The dots are formed between two InP barriers in InAs nanowires with a wurtzite crystal structure which are grown using chemical beam epitaxy. The values of the electron g-factors of the first few electrons entering the dot are found to strongly depend on dot size. They range from close to the InAs bulk value in large dots |g * | = 13 down to |g * | = 2.3 for the smallest dots.PACS numbers: 73.23. Hk, 73.63.Kv, 71.70.Ej The spin of an electron in a quantum dot (QD) is one of the candidates for a scaleable quantum bit, the fundamental unit in quantum computation and quantum communication schemes [1]. Experimental realizations are on the one hand pursued using top-down approaches. This usually involves lateral gate electrodes electrostatically confining few or a single electron in a two dimensional electron gas close to the surface of a Ga(Al)As based heterostructure [2]. Such systems offer good tunability and controlled coupling of multiple spins has been demonstrated [3]. On the other hand, bottom up systems such as self assembled QDs [4] and carbon nanotubes [5] are expected to scale more easily. Semiconductor nanowires have emerged as a promising bottom-up fabricated system for electronic and optical device applications [6]. We have recently demonstrated the creation of few-electron QDs using InAs nanowire heterostructures [7] with two InP barriers. In the following we set out to investigate the spin properties of the first few orbital levels of these QDs.We utilize transport spectroscopy to measure the Zeeman splitting of the energy levels as a function of magnetic field and thereby determine the effective electron g-factor (g * ). The g-factor of bulk InAs, which crystalizes in the zinc-blende (ZB) structure, has been found to be g * = −14.7 [8]. However, InAs nanowires can exhibit both zinc-blende and wurtzite (WZ) type crystal structure[9] depending on diameter and growth conditions and so far very little is known about band parameters in WZ InAs. In low-dimensional semiconductor heterostructures the g factor depends critically on system size and dimensionality [10]. We show that varying the size of our nanowire dots allows us to tune g * from a value close to the InAs bulk value down to |g * | = 2.3±0.3. The possibility to have multiple dots along a nanowire, each with a different g-factor, makes such systems interesting candidates for realizations of individually addressable spin qubits.Using chemical beam epitaxy InAs nanowires containing QDs were grown catalytically from Au nanoparticles deposited on a <111>B InAs substrate [11,12]. The * Electronic address: andreas.fuhrer@ftf.lth.se nanowires typically grow perpendicular to the substrate and high resolution scanning transmission electron microscope (STEM) images indicate that most of them
The electrical and structural properties of 111B-oriented InAs nanowires grown using metal-organic precursors have been studied. On the basis of electrical measurements it was found that the trends in carbon incorporation are similar to those observed in the layer growth, where an increased As/In precursor ratio and growth temperature result in a decrease in carbon-related impurities. Our results also show that the effect of non-intentional carbon doping is weaker in InAs nanowires compared to bulk, which may be explained by lower carbon incorporation in the nanowire core. We determine that differences in crystal quality, here quantified as the stacking fault density, are not the primary cause for variations in resistivity of the material studied. The effects of some n-dopant precursors (S, Se, Si, Sn) on InAs nanowire morphology, crystal structure and resistivity were also investigated. All precursors result in n-doped nanowires, but high precursor flows of Si and Sn also lead to enhanced radial overgrowth. Use of the Se precursor increases the stacking fault density in wurtzite nanowires, ultimately at high flows leading to a zinc blende crystal structure with strong overgrowth and very low resistivity.
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