Advances in quantum technology may come from the discovery of new materials systems that improve the performance or allow for new functionality in electronic devices. Lead telluride (PbTe) is a member of the group IV-VI materials family that has significant untapped potential for exploration. Due to its high electron mobility, strong spin-orbit coupling and ultrahigh dielectric constant it can host few-electron quantum dots and ballistic quantum wires with opportunities for control of electron spins and other quantum degrees of freedom. Here, we report the fabrication of PbTe nanowires by molecular beam epitaxy. We achieve defect-free single crystalline PbTe with large aspect ratios up to 50 suitable for quantum devices. Furthermore, by fabricating a single nanowire field effect transistor, we attain bipolar transport, extract the bandgap and observe Fabry-Pérot oscillations of conductance, a signature of quasiballistic transmission.
We investigate quantum dots in semiconductor PbTe nanowire devices.
Due to the accessibility of ambipolar transport in PbTe, quantum dots
can be occupied both with electrons and holes. Owing to a very large
dielectric constant in PbTe of order 1000, we do not observe Coulomb
blockade which typically obfuscates the orbital and spin spectra. We
extract large and highly anisotropic effective Landé g-factors, in
the range 20-44. The absence of Coulomb blockade allows direct readout,
at zero source-drain bias, of spin-orbit hybridization energies of up to
600 \muμeV.
These spin properties make PbTe nanowires, the recently synthesized
members of group IV-VI materials family, attractive as a materials
platform for quantum technology, such as spin and topological
qubits.
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