Air pollution affects billions of people worldwide, yet ambient pollution measurements are limited for much of the world. Urban air pollution concentrations vary sharply over short distances (≪1 km) owing to unevenly distributed emission sources, dilution, and physicochemical transformations. Accordingly, even where present, conventional fixed-site pollution monitoring methods lack the spatial resolution needed to characterize heterogeneous human exposures and localized pollution hotspots. Here, we demonstrate a measurement approach to reveal urban air pollution patterns at 4-5 orders of magnitude greater spatial precision than possible with current central-site ambient monitoring. We equipped Google Street View vehicles with a fast-response pollution measurement platform and repeatedly sampled every street in a 30-km area of Oakland, CA, developing the largest urban air quality data set of its type. Resulting maps of annual daytime NO, NO, and black carbon at 30 m-scale reveal stable, persistent pollution patterns with surprisingly sharp small-scale variability attributable to local sources, up to 5-8× within individual city blocks. Since local variation in air quality profoundly impacts public health and environmental equity, our results have important implications for how air pollution is measured and managed. If validated elsewhere, this readily scalable measurement approach could address major air quality data gaps worldwide.
Continuous, size resolved particle measurements were performed in two houses in order to determine size-dependent particle penetration into and deposition in the indoor environment. The experiments consisted of three parts: (1) measurement of the particle loss rate following artificial elevation of indoor particle concentrations, (2) rapid reduction in particle concentration through induced ventilation by pressurization of the houses with HEPA-filtered air, and (3) measurement of the particle concentration rebound after house pressurization stopped. During the particle concentration decay period, when indoor concentrations are very high, losses due to deposition are large compared to gains due to particle infiltration. During the concentration rebound period, the opposite is true. The large variation in indoor concentration allows the effects of penetration and deposition losses to be separated by the transient, two-parameter model we employed to analyze the data. For the two houses studied, we found that as particles increased in diameter from 0.1 to 10 µm, penetration factors ranged from ∼1 to 0.3 and deposition loss rates ranged from 0.1 and 5 h −1 . The decline in penetration factor with increasing particle size was less pronounced in the house with the larger normalized leakage area.
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