ÃÃIn this study, the authors considered the effect of soil moisture in the emanation process of radon and thoron gases. Weathered granite soil was selected as the test soil and it was packed in a polypropylene container (275 Â 210 mm 2 and 100 mm in height), up to 50 mm in depth from the bottom. The container was covered with the exhalation rate measuring instrument adopting the accumulation method and -particles were counted at 30 s intervals for 30 min to estimate the exhalation rates. A sporadic increase in the radon and thoron exhalation rates was caused by the increase in the moisture content up to 8%. However, the exhalation rates showed a decreasing tendency with the increase in moisture content over 8%. Although the measured radon exhalation rate was about 25% of the calculated one, both measured and calculated radon exhalation rates had similar trends with an increase in the moisture content in the soil. The measured thoron exhalation rate agreed well with the calculated one. When the moisture content was in the range of 3.5-18%, it was considered that applying the correlation between the moisture content and the measured thoron exhalation rate is useful for estimating the thoron effective diffusion coefficient.
Thoron interference in radon measurements using passive diffusion radon detectors/monitors is a crucial problem when it comes to assessing the internal exposure to radon precisely. The present study reported, as one of the potential factors, the effects of air flow conditions on changes in thoron interference. Rates of thoron infiltration (as thoron interference) into the diffusion chamber of the monitor were evaluated. The temporal variation was obtained based on measurements of the underfloor space of a Japanese wooden dwelling using a diffusion-type radon monitor, a reference radon monitor which was not affected by thoron interference, and a thoron monitor. The thoron infiltration rate for the diffusion-type monitor varied from 0% to 20%. In particular, it appeared to increase when ventilation of the underfloor space air was forced. The variable thoron infiltration rate, with respect to ventilation strength, implied that not only a diffusive process, but also an advective process, played a major role in air exchange between the diffusion chamber of the monitor and the outer air. When an exposure room is characterized by the frequent variation in air ventilation, a variable thoron response is considered to occur in radon–thoron discriminative detectors, in which only diffusive entry is employed as a mechanism for the discrimination of radon and thoron.
An instrument performance test has been carried out for a radon measuring system made in Hungary. The system measures radon using the alpha-track detection technique. It consists of three parts: the passive detector, the etching unit and the evaluation unit. A CR-39 detector is used as the radiation detector. Alpha-track reading and data analysis are carried out after chemical etching. The following subjects were examined in the present study: (1) radon sensitivity, (2) performance of etching and evaluation processes and (3) thoron sensitivity. The radon sensitivity of 6.9 x 10(-4) mm(-2) (Bq m(-3) d)(-1) was acceptable for practical application. The thoron sensitivity was estimated to be as low as 3.3 x 10(-5) mm(-2) (Bq m(-3) d)(-1) from the experimental study.
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