The transient and quasi-steady flame structure of reacting fuel sprays produced by single-hole injectors has been studied using chemiluminescence imaging and Planar Laser-Induced Fluorescence (PLIF) in various constant-volume facilities at different research institutes participating in the Engine Combustion Network (ECN). The evolution of the high-temperature flame has been followed based on chemiluminescence imaging of the excited-state hydroxyl radical (OH *), and PLIF of ground-state OH. Regions associated with low-temperature chemical reactions are visualized using formaldehyde (CH 2 O) PLIF with 355-nm excitation. We compare the results obtained by different research institutes under nominally identical experimental conditions and fuel injectors. In spite of design differences among the various experimental facilities, the results are consistent. This lends confidence to studies of transient behavior and parameter variations performed by individual research groups. We present results of the transient flame structures at Spray A reference conditions, and include parametric variations around this baseline, involving ambient temperature, oxygen concentration and injection pressure. Key results are the observed influence of an entrainment wave on the transient flame behavior, model-substantiated explanations for the high-intensity OH * lobes at the lift-off length and differences with OH PLIF, and a general analogy of the flame structures with a spray cone along which the flame tends to locate for the applied parametric variations.

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A contemporary approach for improving and developing the understanding of heavy-duty Diesel engine combustion processes is to use a concerted effort between experiments at well-characterized boundary conditions and detailed, high-fidelity models. In this paper, combustion processes of n-dodecane fuel sprays under heavy-duty Diesel engine conditions are investigated using this approach. Reacting fuel sprays are studied in a constant-volume pre-burn vessel at an ambient temperature of 900 K with three reference cases having specific combinations of injection pressure, ambient density and ambient oxygen concentration (80, 150 & 160 MPa-22.8 & 40 kg/m 3-15 & 20.5% O 2). In addition to a free jet, two different walls were placed inside the combustion vessel to study flame-wall interaction. Experimentally, low-and high-temperature reaction product distributions are imaged simultaneously using single-shot planar laser-induced fluorescence (PLIF) of formaldehyde and high-speed line-ofsight imaging of the chemically-excited hydroxyl radical (OH*). Interference of soot incandescence in experimental OH* recordings is assessed to improve interpretation of the results. Interference by poly-cyclic aromatic hydrocarbon (PAH) LIF and soot radiation is mostly evaded by evaluating flame structures shortly after ignition for one of the studied cases, but presumably included in others. Simulations were performed using a recently developed computational fluid dynamics (CFD) methodology with detailed chemistry and turbulence-chemistry interaction. Apart from the capability to model flame structures and combustion indicators based on optical diagnostics, heat-release rate trends are predicted accurately at varying boundary conditions. Significant variation in the distribution of low-temperature combustion products under heavy-duty operating conditions are explained using both CFD simulations and a one-dimensional jet model. Fuel pump Resato P16-400-2 Fuel injector Bosch CRI2 solenoid (0.205 mm) Injector driver EFS IPoD 8532 Fuel pressure sensor Kistler 4067E3000 Vessel pressure sensor Kistler 6041 AU20 Burst disk rupture pressure 35 MPa Vessel volume 1260 cc Mixing fan motor Maxon motor (custom) Inlet and exhaust valves Sitec 710.3124-D

The modeling of fuel sprays under well-characterized conditions relevant for heavy-duty Diesel engine applications, allows for detailed analyses of individual phenomena aimed at improving emission formation and fuel consumption. However, the complexity of a reacting fuel spray under heavy-duty conditions currently prohibits direct simulation. Using a systematic approach, we extrapolate available spray models to the desired conditions without inclusion of chemical reactions. For validation, experimental techniques are utilized to characterize inert sprays of n-dodecane in a high-pressure, high-temperature (900 K) constant volume vessel with full optical access. The liquid fuel spray is studied using high-speed diffused back-illumination for conditions with different densities (22.8 and 40 kg/m 3 ) and injection pressures (150, 80 and 160 MPa), using a 0.205-mm orifice diameter nozzle. High-speed Schlieren imaging is used to analyze the influence of these boundary conditions on the spray penetration. Simulations of the fuel spray are performed using a dedicated computational mesh with refinements at the known location of the jet to capture the smallest scales of interest. Using a blob injection model refined with a primary atomization and secondary breakup model, correct trends and good agreement are achieved for both liquid and spray penetration. The capability of capturing the trends at largely varying boundary conditions with a single computational approach provides a solid base for future work.

Multiple-injection strategies are characterized by a complex and transient interplay between high-and low-temperature reactions. Tracking low-temperature reaction products such as formaldehyde (CH2O) is particularly important to understand ignition phenomena and the so-called "combustion recession" that is observed in experiments. Experimentally, it is often difficult to discriminate between formaldehyde and other species such as poly-aromatic hydrocarbons, which is why a selective excitation approach is used in this work. Simultaneous high-speed imaging of the chemicallyexcited hydroxyl radical (OH*) is used to improve indication of flame location and second stage ignition. During experiments in a constant-volume vessel, two 0.5-ms injections of n-dodecane, separated by 0.5-ms dwell time, are injected into a 900-K ambient. The global flame development is characterized based on high-speed diagnostics, followed by an investigation into the spatial distribution of formaldehyde at four different times after start-of-injection (aSOI). Results show significant influence of the first injection on characteristics of the second. Ignition delay and lift-off location of the second injection are prominently reduced, while flame penetration is greatly enhanced by the wake of the first injection. Formaldehyde structure is observed during both end-of-injection transients, reaching as far upstream as 6 mm from the nozzle. Even after the second injection, the flame structure still appears to be influenced by the first, with a shorter lift-off length and compressed formaldehyde structure. Based on the selective excitation procedure, it becomes clear that the interpretation of laser-induced fluorescence (LIF) images obtained by 355-nm excitation alone is prone to ambiguity.