We observe a room-temperature low-threshold transition to a coherent polariton state in bulk GaN microcavities in the strong-coupling regime. Nonresonant pulsed optical pumping produces rapid thermalization and yields a clear emission threshold of 1 mW, corresponding to an absorbed energy density of 29 microJ cm-2, 1 order of magnitude smaller than the best optically pumped (In,Ga)N quantum-well surface-emitting lasers (VCSELs). Angular and spectrally resolved luminescence show that the polariton emission is beamed in the normal direction with an angular width of +/-5 degrees and spatial size around 5 microm.
We report on the current properties of Al1−xInxN (x ≈ 0.18) layers lattice-matched (LM) to GaN and their specific use to realize nearly strain-free structures for photonic and electronic applications. Following a literature survey of the general properties of AlInN layers, structural and optical properties of thin state-of-the-art AlInN layers LM to GaN are described showing that despite improved structural properties these layers are still characterized by a typical background donor concentration of (1–5) × 1018 cm−3 and a large Stokes shift (∼800 meV) between luminescence and absorption edge. The use of these AlInN layers LM to GaN is then exemplified through the properties of GaN/AlInN multiple quantum wells (QWs) suitable for near-infrared intersubband applications. A built-in electric field of 3.64 MV cm−1 solely due to spontaneous polarization is deduced from photoluminescence measurements carried out on strain-free single QW heterostructures, a value in good agreement with that deduced from theoretical calculation. Other potentialities regarding optoelectronics are demonstrated through the successful realization of crack-free highly reflective AlInN/GaN distributed Bragg reflectors (R > 99%) and high quality factor microcavities (Q > 2800) likely to be of high interest for short wavelength vertical light emitting devices and fundamental studies on the strong coupling regime between excitons and cavity photons. In this respect, room temperature (RT) lasing of a LM AlInN/GaN vertical cavity surface emitting laser under optical pumping is reported. A description of the selective lateral oxidation of AlInN layers for current confinement in nitride-based light emitting devices and the selective chemical etching of oxidized AlInN layers is also given. Finally, the characterization of LM AlInN/GaN heterojunctions will reveal the potential of such a system for the fabrication of high electron mobility transistors through the report of a high two-dimensional electron gas sheet carrier density (ns ∼ 2.6 × 1013 cm−2) combined with a RT mobility μe ∼ 1170 cm2 V−1 s−1 and a low sheet resistance, R ∼ 210 Ω/□.
The authors report room temperature polariton lasing at λ∼345nm in a hybrid AlInN∕AlGaN multiple quantum well microcavity (MQW-MC) containing a GaN∕AlGaN MQW active region, i.e., the achievement under nonresonant optical excitation of coherent light emission of a macroscopic population of polaritons occupying the lowest energy state of the lower polariton branch. This was made possible by taking advantage of the efficient relaxation of polaritons in a MQW-MC exhibiting a large vacuum Rabi splitting ΩVRS=56meV.
We observe the build up of strong (∼50%) spontaneous vector polarisation in emission from a GaN-based polariton laser excited by short optical pulses at room temperature. The Stokes vector of emitted light changes its orientation randomly from one excitation pulse to another, so that the timeintegrated polarisation remains zero. This behaviour is completely different to any previous laser. We interpret this observation in terms of the spontaneous symmetry breaking in a Bose-Einstein condensate of exciton-polaritons.PACS numbers: 71.36.+c, 03.75.Kk, Polariton lasers are coherent light sources based on emission of light from a coherent ensemble of excitonpolaritons -the mixed light-exciton quasiparticles in semiconductor microcavities. The concept of polariton lasing was first proposed in 1996 [1], followed a few years later by reports of coherent polariton emission in microcavities [2,3,4]. Recently, we reported polariton lasing at room temperature in GaN-based microcavities [5]. Apart from being very promising for applications, the concept of polariton lasing involves several fundamental physics issues. Contrary to conventional lasers, polariton lasers emit coherent and monochromatic light spontaneously. This is achieved when mixed light-matter quasiparticles (exciton-polaritons), Bosecondense inside a semiconductor microcavity. BoseEinstein condensation (BEC) of the polaritons is a subject of intense experimental and theoretical research at present. Several experimental works claiming polariton BEC have appeared recently [6,7,8]. Though polariton BEC implies polariton lasing these two phenomena are not identical. For polariton lasing a macroscopically populated quantum state of exciton polaritons must be created, which can be considered as a polariton condensate. Polariton lasing does not require thermal equilibrium in the system or the spontaneous build-up of the order parameter, which are the main criteria for BEC when understood as a thermodynamic phase transition. Which experimental measurement should be considered as decisive proof for the exciton-polariton BEC is still a subject of debate within the community. Thermalisation of the exciton-polaritons detected by angle-resolved photoluminescence (PL) measurements has been considered one of the key criteria for a long time [6,7]. However, a similar angular dependence of the PL has also been observed in GaAs-based photon lasers [9]. The spatial coherence of polariton emission demonstrated in Ref.[6] is characteristic for conventional lasers as well. Recent theoretical work suggests that observation of the spontaneous buildup of the vector polarisation in emission from polariton lasers would be evidence for the spontaneous symmetry breaking in the system [10,11,12]. In turn, spontaneous symmetry breaking is considered to be a smoking gun for BEC ever since the pioneering work of Goldstone [13,14].Here we report observations of the build up of the spontaneous vector polarization at room temperature in bulk GaN microcavities. Unlike the recent low temperature e...
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
customersupport@researchsolutions.com
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
This site is protected by reCAPTCHA and the Google Privacy Policy and Terms of Service apply.
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.