We demonstrate a capacitor with high energy densities, low energy losses, fast discharge times, and high temperature stabilities, based on Pb(0.97)Y(0.02)[(Zr(0.6)Sn(0.4))(0.925)Ti(0.075)]O3 (PYZST) antiferroelectric thin-films. PYZST thin-films exhibited a high recoverable energy density of U(reco) = 21.0 J/cm(3) with a high energy-storage efficiency of η = 91.9% under an electric field of 1300 kV/cm, providing faster microsecond discharge times than those of commercial polypropylene capacitors. Moreover, PYZST thin-films exhibited high temperature stabilities with regard to their energy-storage properties over temperatures ranging from room temperature to 100 °C and also exhibited strong charge-discharge fatigue endurance up to 1 × 10(7) cycles.

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We investigated the influence of CuO amount (0.5-3.0 mol%), sintering temperature (900°C-1000°C), and sintering time (2-6 h) on the low-temperature sintering behavior of CuOadded Bi 0.5 (Na 0.78 K 0.22 ) 0.5 TiO 3 (BNKT22) ceramics. Normalized strain (S max /E max ), piezoelectric coefficient (d 33 ), and remanent polarization (P r ) of 1.0 mol% CuO-added BNKT22 ceramics sintered at 950°C for 4 h was 280 pm/V, 180 pC/N, and 28 lC/cm 2 , respectively. These values are similar to those of pure BNKT22 ceramics sintered at 1150°C. In addition, we investigated the performance of multilayer ceramic actuators made from CuO-added BNKT22 in acoustic sound speaker devices. A prototype sound speaker device showed similar output sound pressure levels as a Pb(Zr,Ti)O 3 -based device in the frequency range 0.66-20 kHz. This result highlights the feasibility of using low-cost multilayer ceramic devices made of lead-free BNKT-based piezoelectric materials in sound speaker devices.

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