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To determine the static k (effective neutron multiplication factor) ranging from the critical to an extremely subcritical states, the exponential experiments were performed using various sizes of light-water moderated and reflected low-enriched U0 2 lattice cores. For comparison, the pulsed neutron source experiments were also carried out. In the manner of the Gozani's bracketing method applied to the pulsed source experiment, a formula to obtain k from the measured spatial-decay constant was derived on the basis of diffusion theory. Parameters in the formulas needed to obtain k from the respective experiments were evaluated by 4-group neutron diffusion calculations. The results of the exponential experiments agreed well with those of the pulsed source experiments, the 4-group diffusion calculations and the 137-group Monte Carlo calculations. Therefore, the present data-processing method developed for the exponential experiment was demonstrated to be valid. Besides, through the examination on the parameters used in the data processing, it was found that the dependence of parameter value upon k is weak in the exponential experiment compared with that in the pulsed source experiment. This indicates the superiority of the exponential experiment over the pulsed source experiment for the subcriticality determination of a wide range.

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The reactivity worth of 22.87 grams of 237 Np oxide sample was measured and analyzed in seven uranium cores in the Tank-Type Critical Assembly (TCA) and two uranium cores in the Fast Critical Assembly (FCA) at the Japan Atomic Energy Agency. The TCA cores provided a systematic variation in the neutron spectrum between the thermal and resonance energy regions. The FCA cores, XXI and XXV, provided a hard neutron spectrum of the fast reactor and a soft one of the resonance energy region, respectively. Analyses were carried out using the JENDL-3.3 nuclear data library with a Monte Carlo method for the TCA cores and a deterministic method for the FCA cores. The ratios of calculated to experimental (C/E) reactivity worth were between 0.97 and 0.91, and showed no apparent dependence on the neutron spectrum.

To establish a technique of on-site subcriticality determination suitable for the criticality safety management of nuclear fuel assembly, the applicability of the method proposed by Mihalczo was examined with the Tank-type Critical Assembly (TCA) of the Japan Atomic Energy Research Institute. In the Mihalczo method, cross power spectral densities and auto power spectral densities are evaluated from the output currents of an ionization chamber containing 252Cf neutron source and two neutron detectors. The principle of this method is that the spectral ratio formed by the power spectral densities mentioned can be related to the subcriticality by the help of a stochastic theory.Throughout our data processing, an improved formula taking account of the neutron extinction at a detection process was used. Up to the subcriticality of 15 dollars, the Mihalczo method agreed with the water-level worth method, which has been a standard method of reactivity determination at the TCA facility. The systems treated in the present report hold symmetry concerning the nuclear fuel configuration and the 252Cf chamber position. It was clarified that, contrary to Mihalczo's assertion, the factor converting the spectral ratio to a subcriticality depends on subcriticality itself.