We experimentally investigate and quantitatively analyze the spin Hall magnetoresistance effect in ferromagnetic insulator/platinum and ferromagnetic insulator/nonferromagnetic metal/platinum hybrid structures. For the ferromagnetic insulator, we use either yttrium iron garnet, nickel ferrite, or magnetite and for the nonferromagnet, copper or gold. The spin Hall magnetoresistance effect is theoretically ascribed to the combined action of spin Hall and inverse spin Hall effect in the platinum metal top layer. It therefore should characteristically depend upon the orientation of the magnetization in the adjacent ferromagnet and prevail even if an additional, nonferromagnetic metal layer is inserted between Pt and the ferromagnet. Our experimental data corroborate these theoretical conjectures. Using the spin Hall magnetoresistance theory to analyze our data, we extract the spin Hall angle and the spin diffusion length in platinum. For a spin-mixing conductance of 4 × 10 14 −1 m −2 , we obtain a spin Hall angle of 0.11 ± 0.08 and a spin diffusion length of (1.5 ± 0.5) nm for Pt in our thin-film samples.
We report on spin Hall magnetoresistance (SMR) measurements of Pt Hall bars on the antiferromagnetic NiO(111) single crystal. An SMR with a sign opposite of conventional SMR is observed over a wide range of temperatures as well as magnetic fields stronger than 0.25T. The negative sign of the SMR can be explained by the alignment of magnetic moments being almost perpendicular to the external magnetic field within the easy plane (111) of the antiferromagnet. This correlation of magnetic moment alignment and external magnetic field direction is realized just by the easy-plane nature of the material without the need of any exchange coupling to an additional ferromagnet. The SMR signal strength decreases with increasing temperature, primarily due to the decrease in Néel order by including fluctuations. An increasing magnetic field increases the SMR signal strength as there are less domains and the magnetic moments are more strongly manipulated at high magnetic fields. The SMR is saturated at an applied magnetic field of 6 T resulting in a spin-mixing conductance of ∼ 10 18 Ω −1 m −2 , which is comparable to that of Pt on insulating ferrimagnets such as yttrium iron garnet. An argon plasma treatment doubles the spin-mixing conductance.
We studied the nonlocal transport behavior of both electrically and thermally excited magnons in yttrium iron garnet (YIG) as a function of its thickness. For electrically injected magnons, the nonlocal signals decrease monotonically as the YIG thickness increases. For the nonlocal behavior of the thermally generated magnons, or the nonlocal spin Seebeck effect (SSE), we observed a sign reversal which occurs at a certain heater-detector distance, and it is influenced by both the opacity of the YIG/heater interface and the YIG thickness. Our nonlocal SSE results can be qualitatively explained by the bulk-driven SSE mechanism together with the magnon diffusion model. Using a two-dimensional finite element model (2D-FEM), we estimated the bulk spin Seebeck coefficient of YIG at room temperature. The quantitative disagreement between the experimental and modeled results indicates more complex processes going on in addition to magnon diffusion and relaxation, especially close to the contacts.
The spin polarization of Pt in Pt/NiFe2O4 and Pt/Fe bilayers is studied by interface-sensitive x-ray resonant magnetic reflectivity to investigate static magnetic proximity effects. The asymmetry ratio of the reflectivity was measured at the Pt L3 absorption edge using circular polarized x-rays for opposite directions of the magnetization at room temperature. The results of the 2% asymmetry ratio for Pt/Fe bilayers are independent of the Pt thickness between 1.8 and 20 nm. By comparison with ab initio calculations, the maximum magnetic moment per spin polarized Pt atom at the interface is determined to be (0.6 ± 0.1) µB for Pt/Fe. For Pt/NiFe2O4 the asymmetry ratio drops below the sensitivity limit of 0.02 µB per Pt atom. Therefore, we conclude, that the longitudinal spin Seebeck effect recently observed in Pt/NiFe2O4 is not influenced by a proximity induced anomalous Nernst effect. In spintronics1 and spin caloritronics 2 pure spin currents can be generated in ferromagnetic insulators (FMIs) by spin pumping 3 , the spin Hall effect 4 and the spin Seebeck effect 5 . Since these spin currents play an important role in spintronic applications, an understanding of the generation, manipulation and detection of spin currents is an important topic of research. A common spin current detection technique uses a nonferromagnetic metal (NM) thin film grown on a ferromagnet (FM). The inverse spin Hall effect 6 converts the spin current into a transverse voltage in the NM. Pt is commonly used as NM due to its large spin Hall angle 7 , but has generated some controversy in the interpretation because of its closeness to the Stoner criterion, which can induce, e.g., Hall or Nernst effects due to the proximity to the FM 8 .For a quantitative evaluation of the spin Seebeck effect (thermal generation of spin currents) one has to exclude or separate various parasitic effects. It is reported 5 that in transverse spin Seebeck experiments a spin current is generated perpendicular to the applied temperature gradient which is typically aligned in-plane. For ferromagnetic metals (FMMs) with magnetic anisotropy, the planar Nernst effect 9 can contribute 10 due to the anisotropic magnetothermopower. Furthermore, out-of-plane temperature gradients due to heat flow into the surrounding area 11 or through the electrical contacts 12 can induce an anomalous Nernst effect (ANE) [13][14][15] or even an unintended longitudinal spin Seebeck effect as recently reported 16 .The longitudinal spin Seebeck effect (LSSE) 17 describes a spin current that is generated parallel to the temperature gradient, which is typically aligned outof-plane to drive the parallel spin current directly into the NM material. For FMMs or semiconducting ferromagnets an ANE can also contribute to the measured voltage 18 . Furthermore, for NM materials close to the Stoner criterion a static magnetic proximity effect in the NM at the NM/FMI interface can lead to a proximity induced ANE 8 . If an in-plane temperature gradient is applied, a proximity induced planar Nernst effect ...
Transverse magnetothermoelectric effects are studied in Permalloy thin films grown on MgO and GaAs substrates and compared to those grown on suspended SiN(x) membranes. The transverse voltage along platinum strips patterned on top of the Permalloy films is measured versus the external magnetic field as a function of the angle and temperature gradients. After the identification of the contribution of the planar and anomalous Nernst effects, we find an upper limit for the transverse spin Seebeck effect, which is several orders of magnitude smaller than previously reported.
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