In this paper, we present an investigation on the use of Au-Ag alloy popcorn-shaped nanoparticles (NPs) to realise the broadband optical absorption enhancement of dye-sensitized solar cells (DSCs). Both simulation and experimental results indicate that compared with regular plasmonic NPs, such as nano-spheres, irregular popcorn-shaped alloy NPs exhibit absorption enhancement over a broad wavelength range due to the excitation of localized surface plasmons (LSPs) at different wavelengths. The power conversion efficiency (PCE) of DSCs is enhanced by 16% from 5.26% to 6.09% by incorporating 2.38 wt% Au-Ag alloy popcorn NPs. Moreover, by adding a scattering layer on the exterior of the counter electrode, the popcorn NPs demonstrate an even stronger ability to increase the PCE by 32% from 5.94% to 7.85%, which results from the more efficient excitation of the LSP mode on the popcorn NPs.
In this paper, the energy-time entangled photon-pairs at 1.5 μm are generated by the spontaneous four wave mixing (SFWM) in optical fibers under continuous wave (CW) pumping. The energy-time entanglement property is demonstrated experimentally through an experiment of Franson-type interference. Although the generation rates of the noise photons are one order of magnitude higher than that of the photon-pairs under CW pumping, the impact of noise photons can be highly suppressed in the measurement by a narrow time domain filter supported by superconducting nanowire single photon detectors with low timing jitters and time correlated single photon counting (TCSPC) module with high time resolution. The experiment results show that the SFWM in optical fibers under CW pumping provides a simple and practical way to generate energy-time entanglement at 1.5 μm, which has great potential for long-distance quantum information applications over optical fibers.
In this Letter, telecom-band degenerate-frequency photon pairs are generated in a specific mode of a silicon microring cavity by the nondegenerate spontaneous four-wave mixing (SFWM) process, under two continuous-wave pumps at resonance wavelength of two different cavity modes. The ratio of coincidence to accidental coincidence is up to 100 under a time bin width of 5 ns, showing their characteristics of quantum correlation. Their quantum interference in balanced and unbalanced Mach-Zehnder interferometers is investigated theoretically and experimentally, and the results show potential in quantum metrology and quantum information.
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