2022
DOI: 10.26434/chemrxiv-2022-f362k
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Concentration-dependent characteristics of a complex coacervate

Abstract: In this work, we have comprehensively and systematically investigated the influence of the initial concentration of oppositely charged polyelectrolyte solutions on the interaction strength, interfacial tension and local structure of the coacervate phase generated at charge stoichiometry in a PDADMAC/PANa model system. We have shown for the first time that the concentration has a direct and significant impact on the complexation strength between the two polyelectrolytes, leading to lighter coacervates with cons… Show more

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