“…It is well-known that the chemical, physical, and mechanical properties of nanomaterials are associated with their shapes, aspect ratios, as well as elemental compositions, whereas their final properties mainly depend on the synthesis process. , For this reason, a variety of processes leading to the formation of magnetic metallic as well as alloy-type one-dimensional nanostructures have been successfully developed so far, including lithography, , laser-assisted deposition techniques, , chemical vapor deposition (CVD), , thermal decomposition, − and hydrothermal or solvothermal syntheses. ,− However, the most frequently applied method to produce wire-like nanomaterials is a template-assisted electrochemical synthesis. − ,,,,− This is mainly associated with the fact that this process is based on a very simple approach in which the reduction of the required material occurs in the pores of the template due to the application of electrochemical procedures. This leads to the formation of simple, single metal wire-like structures ,, as well as more complex binary or ternary metal nanoalloys with desired compositions. ,,,− Furthermore, this technique allows control of diameters, lengths, and distances between wire-like structures by adjusting pore diameter, pore depth, and distance between pores, respectively. ,, On the other hand, the template-assisted electrochemical deposition is typically a multistep process leading to the formation of low quantity of material, and at the time, it is quite difficult to remove as-formed wire-like structures from matrices without damaging or modification of their surfaces. ,,,,, Hence, even if this method is good for manufacturing complex wire-like structures like binary or ternary nanoalloys, it is not convenient for application in large-scale production.…”