“…The free energy of formation of amorphous SiO, has been adjusted with respect to that given in ref. 20 in order to account for the relative observed solubilities of amorphous SiO, and ~ 2 3 The resulting database was then found to give acceptable agreement with experimental data for the solubility of amorphous SiO, as a function of pH and the solubility of portlandite. For example the pH and [Call for portlandite in water at 25 "C were calculated to be 12.41 and 0.0225 respectively, whereas the corresponding measured values are 12.45 and 0.0203.…”