2018
DOI: 10.1364/ol.43.001403
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Stimulated Raman spectroscopy of analytes evanescently probed by a silicon nitride photonic integrated waveguide

Abstract: We report, to the best of our knowledge, the first demonstration of stimulated Raman spectroscopy enhanced by a nanophotonic integrated circuit. The Raman response of low-concentration dimethyl sulfoxide is evanescently probed via centimeter-long wire waveguides. A signal enhancement of close to five orders of magnitude, as compared to the case of on-chip spontaneous Raman scattering, is demonstrated. This significant enhancement factor allows for the use of continuous-wave lasers with milliwatt-level power an… Show more

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Cited by 41 publications
(25 citation statements)
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“…Our approach can be readily extended to efficiently determine optimal waveguide geometries for other sensing modes, such as stimulated Raman spectroscopy [81], with a suitably defined sensing metric. There are also a number of other material platforms to which this work can be extended, such as silicon nitride on silicon dioxide [33,34,82,83], titanium dioxide on silicon dioxide [35], chalcogenide glass on insulator [84,85], germanium or germaniumsilicon on silicon [86,87], silicon on sapphire [88], and more that are of great interest to the waveguide-integrated chemical sensing community.…”
Section: Discussionmentioning
confidence: 99%
“…Our approach can be readily extended to efficiently determine optimal waveguide geometries for other sensing modes, such as stimulated Raman spectroscopy [81], with a suitably defined sensing metric. There are also a number of other material platforms to which this work can be extended, such as silicon nitride on silicon dioxide [33,34,82,83], titanium dioxide on silicon dioxide [35], chalcogenide glass on insulator [84,85], germanium or germaniumsilicon on silicon [86,87], silicon on sapphire [88], and more that are of great interest to the waveguide-integrated chemical sensing community.…”
Section: Discussionmentioning
confidence: 99%
“…This waveguide based excitation and collection technique can be used for different sensing phenomena e.g. on-chip fluorescence [1], spontaneous Raman [2], stimulated Raman [3] and surface enhanced Raman spectroscopy [4], whereby unlike confocal approaches, the signal scales with the waveguide length. Different photonic structures i.e.…”
Section: Introductionmentioning
confidence: 99%
“…Typical PON systems have two wavelengths near 1310 and 1490/ 1550 nm required for upstream and downstream signals channeling, which requires the photonic integrated circuit to perform dual-wavelength-band coupling and duplexing. Other applications may include on-chip amplification by coupling pump and signal lights simultaneously and integrated Raman spectrometry [ 96 , 97 ].…”
Section: Polarization and Wavelength Diversitymentioning
confidence: 99%