In this work, we investigate the Molecular-Frame Photoelectron Momentum and Angular Distributions (MF-PMD and MF-PAD) of H$^+_2$ in the presence of XUV Attosecond Pulses. We present the sensitive alignment effect of MF-PMD and MF-PADs when the laser field polarization and the molecular axis are close to parallel geometry. Results show that the MF-PADs and MF-PMDs of single-photon single ionization of H$^+_2$ ion dramatically change when the alignment slightly shifts from parallel geometry to a small alignment angle (e.g., 1$^{\circ}$) between laser polarized direction and the molecular axis with equilibrium inter-nuclear distance R$_c$=2. As the R$_c$ increase to 4, such sensitivity is decreased. The inter-nuclear distance-dependent transition cross-section to different channels is found to be the origin of such sensitivity.

We perform a theoretical study on dynamic interference in single photon ionization of ground state hydrogen atoms in the presence of a super-intense ultra-fast chirped laser pulse of different chirp types (equal-power and equal-FWHM laser pulses) by numerically solving the time-dependent Schrödinger equation in one dimension. We investigate the influences of peak intensity and chirp parameters on the instantaneous ionization rate and photoelectron yield, respectively. We also compare the photoelectron energy spectra for the ionization by the laser pulses with different chirp types. We find that the difference between the instantaneous ionization rates for the ionization of hydrogen atom driven by two different chirped laser pulses is originated from the difference in variation of vector potentials with time.

We use a numerically solved time-dependent Schrödinger equation for calculating the photoelectron momentum distribution of ground-state hydrogen atoms in the presence of superintense ultrashort high-frequency pulses. It is demonstrated that the dynamic interference effect within a superintense XUV laser beam has the ability to significantly alter the photoelectron momentum distribution. In our work, a clearly visible dynamic interference pattern is observed when hydrogen atoms are exposed to a superintense circularly polarized laser pulse with a photon energy of ℏω = 53.605 eV, which has previously been found for linearly polarized pulses or the weakly bounded model H− system for circularly polarized pulses. Angular-distorted interference arises for linear superintense XUV pulses of similar intensity. The significant differences in photoelectron momentum distributions that have been seen by linearly and circularly polarized XUV pulses are caused by the Coulomb rescattering phenomenon.

We examine conditions under which an open quantum system composed of a driven degenerated parametric oscillator cavity and a driven two-level atom coupled to a waveguide could decay to a pure dark state rather than the expected mixed state. The calculations are carried out analytically in a low dimensional Hilbert space truncated at the double-excitation states of the combined system. The validity of the truncation is confirmed by the exact numerical analysis. It is found that one way to produce the pure state is to chirally couple the cavity and the atom to the waveguide. Another way to produce the pure state is to drive the cavity and the atom with unequal detunings. In both cases, if the driving fields are weak, the produced state is a coherent superposition of only the single-excitation and ground states of the combined system. In addition, we have found a direct correspondence between the generation of the dark state and the photon blockade effect. In other words, the generation of the dark state acts as a blockade to the number of photons so that only a single photon can be present in the cavity. We investigate the normalized second-order correlation function of the cavity field and find that the conditions under which the correlation function vanishes coincide with the conditions for the creation of the pure dark state. This system is, therefore, suggested as an alternative scheme for the generation of single-photon states.Comment: published versio

We investigate the intensity effect of ultrashort assisting infrared laser pulse on the single-XUV-photon double ionization of helium atoms by solving full six-dimensional time-dependent Schrödinger equation with implement of finite element discrete variable representation. The studies of joint energy distributions and joint angular distributions of the two photoelectrons reveal the competition for ionized probabilities between the photoelectrons with odd parity and photoelectrons with even parity in single-XUV-photon double ionization process in the presence of weak infrared laser field, and such a competition can be modulated by changing the intensity of the weak assisting-IR laser pulses. The emission angles of the two photoelectrons can be adjusted by changing the laser parameters as well. We depict how the assisting-IR laser field enhances and/or enables the back-to-back and side-by-side emission of photoelectrons created in double ionization process.