The resistance of the electron gas (2DEG) at the interface between the two band insulators LaAlO3 (LAO) and SrTiO3 (STO) typically drops monotonically with temperature and R/T curves during cooling and warm-up look identical for large area structures. Here we show that if the LAO/STO is laterally restricted by nanopatterning the resistance exhibits a temperature anomaly. Warming up nanostructures from low temperatures leads to one or two pronounced resistance peaks between 50 and 100 K not observed for larger dimensions. During cool-down current filaments emerge at the domain walls that form during a structural phase transition of the STO substrate. During warm-up the reverse phase transition can interrupt filaments before the sheet conductivity which dominates at higher temperature is reestablished. Due to the limited number of filaments in a nanostructure this process can result in a complete loss of conductance. As a consequence of these findings the transport physics extracted from experiments in small and large area LAO/STO structures may need to be reconsidered.
We report the fabrication of nanostructures from the quasi-two-dimensional electron gas (q2DEG) formed at the LaAlO3/ SrTiO3 (LAO/STO) interface. The process uses electron beam lithography in combination with reactive ion etching. This technique allows to pattern high-quality structures down to lateral dimensions as small as 100nm while maintaining the conducting properties without inducing conductivity in the STO substrate. Temperature dependent transport properties of patterned Hall bars of various widths show only a small size dependence of conductivity at low temperature as well as at room temperature. The deviation can be explained by a narrow lateral depletion region. All steps of the patterning process are fully industry compatible.
As spintronic devices become more and more prevalent, the desire to find Pt-free materials with large spin Hall effects is increasing. Previously it was shown that β-W, the metastable A15 structured variant of pure W, has charge-spin conversion efficiencies on par with Pt, and it was predicted that β-W/Ta alloys should be even more efficient. Here we demonstrate the enhancement of the spin Hall ratio (SHR) in A15-phase β-W films doped with Ta (W4-xTax where 0.28 <= x <= 0.4) deposited at room temperature using DC magnetron co-sputtering. In close agreement with theoretical predictions, we find that the SHR of the doped films was ~9% larger than pure -W films. We also found that the SHR's in devices with Co2Fe6B2 were nearly twice as large as the SHR's in devices with Co4Fe4B2. This work shows that by optimizing deposition parameters and substrates, the fabrication of the optimum W3Ta alloy should be feasible, opening the door to commercially viable, Pt-free, spintronic devices. Introduction/Background:Recently, the spin Hall effect (SHE) has received a great deal of attention not only from a fundamental physics perspective but also for technological applications in the area of memories, logic and sensors[1][2]. The SHE is the conversion of a longitudinal current density into a transverse spin current density, which is characterized by the spin Hall ratio (SHR), θSH=JS/JC and materials with large SHRs are desired for spintronic applications. Note that SHR and SHA (spin Hall angle) have been used interchangeably in literature, however the SHA is rigorously defined as the tan -1 (JS/JC). Previous studies have demonstrated only a handful of materials that can be sputter-deposited and which exhibit large SHRs at room temperature: these include Pt/doped Pt [3], β-Ta [4], β-W [5] and oxygen doped β-W [6]. There is a technological desire towards Pt-free spintronics and among these candidates, β-W and oxygen doped β-W, have the highest resistance (resulting in larger power requirements) but also show the largest SHR, which is approximately -0.35 and -0.5, respectively [5][6][7] [8]. β-W is a metastable phase of W that exhibits the cubic A15 structure (SG# 223, Pm-3n) which has two distinct crystallographic sites with two atoms located on each face of the cubic cell. The α-W phase, on the other hand, is the most stable form of W that crystallizes in body centered cubic structure, while exhibiting a smaller SHE
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