2015
DOI: 10.1002/adma.201501888
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Graphene Quantum Dots Doping of MoS2 Monolayers

Abstract: Graphene quantum dots (GQDs) interacting with molybdenum disulfide (MoS2 ) monolayers induce an effective photoexcited charge transfer at the interface. Both the photoluminescence (PL) and valley polarization of this GQDs/MoS2 heterostructure can be modulated under various doping charge densities. The photon-exciton interaction is used to explain and calculate the heterostructure PL control, and is further applied to the valley-polarization tuning.

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Cited by 175 publications
(186 citation statements)
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“…On the contrary, plasmonics enable strong light-matter interaction with 2D materials due to high field concentration [135][136][137][138]. Additionally, it has been shown that surface plasmons in metallic nanoparticles can directly interact with 2D materials through hot electron injection [42,[139][140][141][142][143]. For instance, hot electrons can change the doping of graphene [140] or molybdenum disulfide (MoS 2 ) [42,143], leading to structural phase transitions [42] or modulation of the absorption spectrum [143].…”
Section: Hot Electrons With 2d Materialsmentioning
confidence: 99%
“…On the contrary, plasmonics enable strong light-matter interaction with 2D materials due to high field concentration [135][136][137][138]. Additionally, it has been shown that surface plasmons in metallic nanoparticles can directly interact with 2D materials through hot electron injection [42,[139][140][141][142][143]. For instance, hot electrons can change the doping of graphene [140] or molybdenum disulfide (MoS 2 ) [42,143], leading to structural phase transitions [42] or modulation of the absorption spectrum [143].…”
Section: Hot Electrons With 2d Materialsmentioning
confidence: 99%
“…The drain–source current is controlled by the gate voltage on the dielectric layer. High carrier mobility, high switching ratio and low subthreshold swing means high performance FET, which depends on the metal contacts,247 channel materials (thickness,248, 249 doping,192, 250, 251, 252, 253, 254 heterostructures200, 208), dielectric materials (back‐gate,86, 255 top‐gate,256 liquid gate257), and so forth. 2D GIVMCs based FETs have demonstrated exciting performance.…”
Section: Device Applicationsmentioning
confidence: 99%
“…The absorption and recombination of excitons directly affect the light absorption and luminescence of semiconductors. In 2D semiconductor materials [63][64][65][66] , due to their low dimensionality and surface defects, the spatial resolution must be reduced to the nanometer scale in order to study exciton recombination and optical properties. However, the traditional photoluminescence is restricted at sub-nanoscale due to the diffraction limit of incident light.…”
Section: Microscopy For Semiconductorsmentioning
confidence: 99%