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One-dimensional (1D) conductive nanowire is one of the most important components for the development of nanosized electronic devices, sensors, and energy storage units. Great progresses have been made to prepare the 1D-conducting polymeric nanofibers by the low concentration process or the synthesis with hard or soft templates. However, it still remains as a great challenge to prepare polymeric nanofibers with narrow dispersity, high aspect ratio, and good processibility. With the rod-like tobacco mosaic virus as the template, 1D-conducting polyaniline and polypyrrole nanowires can be readily prepared via a hierarchical assembly process. This synthesis discloses a unique way to produce composite fibrillar materials with controlled morphology and great processibility, which can promote many potential applications including electronics, optics, sensing, and biomedical engineering.
A new chemical sensor based on reverse-biased graphene/Si heterojunction diode has been developed that exhibits extremely high bias-dependent molecular detection sensitivity and low operating power. The device takes advantage of graphene's atomically thin nature, which enables molecular adsorption on its surface to directly alter graphene/Si interface barrier height, thus affecting the junction current exponentially when operated in reverse bias and resulting in ultrahigh sensitivity. By operating the device in reverse bias, the work function of graphene, and hence the barrier height at the graphene/Si heterointerface, can be controlled by the bias magnitude, leading to a wide tunability of the molecular detection sensitivity. Such sensitivity control is also possible by carefully selecting the graphene/Si heterojunction Schottky barrier height. Compared to a conventional graphene amperometric sensor fabricated on the same chip, the proposed sensor demonstrated 13 times higher sensitivity for NO₂ and 3 times higher for NH₃ in ambient conditions, while consuming ∼500 times less power for same magnitude of applied voltage bias. The sensing mechanism based on heterojunction Schottky barrier height change has been confirmed using capacitance-voltage measurements.
The efficiency of multi‐layer OLEDs using indium tin oxide (ITO) and triphenyldiamine is limited by the hole injection rate, or the quality of the contact between the two components, respectively. Coating the ITO with an ultra‐thin Pt layer dramatically improves hole injection, and significantly lowers the devices' operating voltage. The Figure juxtaposes AFM images of an unmodified (left) and Pt‐coated ITO electrode (right).
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