Efficient sources of individual pairs of entangled photons are required for quantum networks to operate using fiber-optic infrastructure. Entangled light can be generated by quantum dots (QDs) with naturally small fine-structure splitting (FSS) between exciton eigenstates. Moreover, QDs can be engineered to emit at standard telecom wavelengths. To achieve sufficient signal intensity for applications, QDs have been incorporated into one-dimensional optical microcavities. However, combining these properties in a single device has so far proved elusive. Here, we introduce a growth strategy to realize QDs with small FSS in the conventional telecom band, and within an optical cavity. Our approach employs ''droplet-epitaxy'' of InAs quantum dots on (001) substrates. We show the scheme improves the symmetry of the dots by 72%. Furthermore, our technique is universal, and produces low FSS QDs by molecular beam epitaxy on GaAs emitting at ∼900 nm, and metal-organic vapor-phase epitaxy on InP emitting at ∼1550 nm, with mean FSS 4× smaller than for Stranski-Krastanow QDs.
The measurement of ζ potential of Ga-face and N-face gallium nitride has been carried out as a function of pH. Both of the faces show negative ζ potential in the pH range 5.5–9. The Ga-face has an isoelectric point at pH 5.5. The N-face shows a more negative ζ potential due to larger concentration of adsorbed oxygen. The ζ potential data clearly showed that H-terminated diamond seed solution at pH 8 will be optimal for the self-assembly of a monolayer of diamond nanoparticles on the GaN surface. The subsequent growth of thin diamond films on GaN seeded with H-terminated diamond seeds produced fully coalesced films, confirming a seeding density in excess of 10 11 cm –2 . This technique removes the requirement for a low thermal conduction seeding layer like silicon nitride on GaN.
Optical transmittance measurements on epitaxial, phase-pure, wurtzite-structure Sc x Ga 1-x N films with 0 ≤ x ≤ 0.26 showed that their direct optical band gaps increased from 3.33 eV to 3.89 eV with increasing x, in agreement with theory. These films contained I 1 -and I 2 -type stacking faults. However, the direct optical band gaps decreased from 3.37 eV to 3.26 eV for Sc x Ga 1-x N films which additionally contained nanoscale lamellar inclusions of the zincblende phase, as revealed by aberration-corrected scanning transmission electron microscopy. Therefore we conclude that the apparent reduction in Sc x Ga 1-x N band gaps with increasing x is an artefact resulting from the presence of nanoscale zinc-blende inclusions.
Semiconductor quantum dots embedded in hybrid circular Bragg gratings are a promising platform for the efficient generation of nonclassical light. The scalable fabrication of multiple devices with similar performance is highly desirable for their practical use as sources of single and entangled photons, while the ability to operate at telecom wavelength is essential for their integration with the existing fiber infrastructure. In this work, we combine the promising properties of broadband hybrid circular Bragg gratings with a membrane-transfer process performed on 3 in. wafer scale. We develop and characterize single-photon sources based on InAs/GaAs quantum dots emitting in the telecom O-band, demonstrating bright single-photon emission with Purcell factor >5 and count rates up to 10 MHz. Furthermore, we address the question of reproducibility by benchmarking the performance of 10 devices covering a wide spectral range of 50 nm within the O-band.
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